INTRRNAL DEPOSITION OF RADIONUCLIDES nord the amatyss ot 4 months represents only radielagical deray. Thas, the results are net directly camparsble te those obtained from ani- mals which were returned alive, and in which belagical turnever se well as radiologyal decay were operating. The largest fraction of the grom beta activity In two of the fish in which bones and muscle were sep- + AUPE SRI arated and analysed, equal amonnts of activity were found in each fraction. However, the storage of these fish in formaldehyde for 3 months may have permitted the diffusion of the radioelements from bone to muscle to take place. Further studies on fresh fish will clarify nae nal) enbintnn, this point. The contamination of the fish in the lagoon was considerably greater than that of the land animals studied. As tish form a large staple item in the diet of the Marshallese, the high level of contamination is important. At the end of a 214-month experimental! period. the excretion by the chickens of both bets and gamma activity per 24 hours was 5 percent of the value measured at the start at 37 days post detonation (Fig. 5.1). Analysis of pig excreta indicated a similar decrease of activity with time. In a 6-week period, the yamma activity excreted per 24 hours decreased to about 2.5 percent of the activity excreted at 44 days post detonation. The excreta of the pigs from Utirik contained less than 10 percent of the gross beta activity found in the excreta of the pigs from Rongelap at the same time. This ratio of 1 was approx. imately the same ratio found between the activity of the food, water and soil samples of the two locations, Radiochemtral Analysia of Tissues and Erereta. Radiochemical analysis of pig tissues indicated that t2 percent of the skeletal beta activity was derived from Se. 7 percent from Bal. and 10 percent from the rare earth group at *Z days post detonation (Table “.3). The radioisotopic composition of the urine at this time was simular to that of the skeleton, The distribution of activity in the body of the pig Ca ee to ee te TDSSToe wy represeat the distribution in hamen bemgs. The sheolute amount of internal contannnetion m the Rongelap people was, however, only s tenth of that fownd in the animals. At 4 months pest detonation, the atkaies eerie compris ieee thai 2 p<corent of the tated activity in the clam (Table 5.10). The rece in the fek was contributed by the concentragon of radioactive material in the viscera. 8i earth growp constituted 43 percent of the total beta activity. The balance of the activity was contributed chiefly by Zr’* (2! percent) and Ru'*'* (32 percent). About 50 percent of the material found in the viscera of the fish was of the rare earth group. Very small amounts of strontium and barium were found. In the tissues of the fish, strontium, barium and the rare earths contributed only about 10 percent of the total activity. 5.43 Autoradiographs A number of autoradiographs of the tibiae and femurs of | chick, 4 pigs, 1 rooster and 2 chickens were prepared beth at the USNRDL and at the Argonne National Laboratory (ANIL) to determine the pattern of deposition of fission products. Contact printaing on X-ray no-sereen film was found to be the most satifactory method of preparing the autoradiographs. The discussion and conclusions presented below summarize the tindings reported by Norris (15). The autoradiograph of a tibia from a chicken sacrificed at 45 days post detonation (Fig. 5.2) indicated a relatively uniform distmbution of the activicy throughout most of the bone, with the highest concentration of activity in the area adjacent to the epiphysis. This area of high uvtivity corresponds to an area of dense trabecular bone. The tibia and femur of a baby chick, which died spontaneously 47 days post: detonation, showed the heaviest concentranion of radioactive material in the diaphysir (Fig. 5.3). The end regions of the bone, which were laid down after the animals were removed from the cuntaminated environment, were relatively lacking Inactivity. The region of greatest activity was mothe dinphysis, which appeared to be ab- es es: tne > ee oreee poe Soe ee meme nn nee ee

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