in the stainless steel. The instrument response is energy dependent, and data
from the manufacturer indicate an error of as much as 6 to 10% could result if

energy corrections are not made to the gross readings®.,

The RSS~11lls used in this study were calibrated at the factory against radium sources whose calibration is traceable to the National Bureau of Standards.
The calibration of the instruments was also checked at the Environmental

Monitoring Laboratory (formerly Health and Safety Laboratory) before and after
field use.

In the report on external exposure for all other atolls surveyed by BNL3,
energy dependence corrections were calculated for data from Rongelap and
Rongerik Atolls. The factors needed to compensate the RSS~111 response for

energy dependence ranged from 1.01 to 1.05.
mately 1.02.

B)

The mean correction was approxi-

Thermoluminescent Survey
Lithium fluoride (LiF) thermoluminescent dosimeter chips 1/4~-inch square

were used>, for several reasons. LiF is approximately a tissue equivalent material, and its response is essentially energy independent for photon energies
greater than 20 keV up to several MeV. The system is precise to 2% and has a
long term retention of 5% loss at room temperature for one year. These
qualities made the LiF ideal for use in the Marshall Islands.
All TLDs were cleaned with analytical grade methanol before departure for
the Marshall Islands and prior to analysis. Prior to irradiation, the TLDs were
annealed at 400°C for one hour and them at 100°C for 2 hr. After field exposure
and before reading, the TLDs were annealed at 100°C for 10 min.
In addition to the TLDs exposed in the field at Bikini and Eneu, several
sets of TLDs were assembled for use in correcting field measurements for back~
ground, fading and air transportation contributions.
Several TLDs were annealed
and then immediately stored in a lead pig in the BNL analytical counting area.
An equal number of TLDs were irradiated to 100 mR and stored with the background
TLDs to determine fading losses. Four other TLDs were sent to Kwajalein and
stored there in a lead pig to determine in-transit contributions to the response. All TLD results have been corrected for these parameters.
The TLDs were calibrated at BNL with !37Cs gamma and 90sr/90y betas.

Re-

sults are directly related to the external exposure and beta absorbed dose that

would be received by individuals living on Bikini and Eneu Islands.

Because the total response must be differentiated into beta and gamma
components, a TLD holder was developed that would eliminate nearly 100% of the
90Y beta of 2.27 MeV (Figure 1). Four TLDs are used per holder. Two are
covered by 1100 mg/cm? of aluminum and Mylar which is of sufficient mass density
thickness to eliminate beta response; these provide the gamma response.
The two
other TLDs are shielded by “ 15 mg/cm? Mylar to respond to the total gamma~beta

contribution at one meter above the earth's surface.

The difference between the

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