162 DREVINSKY AND PECCI Table 1—SAMPLING DATA FOR IMPACTOR-FILTER COLLECTIONS Flight No. Sampling Tropopause interval, km km altitude —Date 9.1 to 14.4 height, 2576 Mar. 16,1962 2606 Sept. 25,1962 9.1 15.2 21.3 27.4 15.2 21,3 27.4 29.6 10.5 2617 May 16, 1963 9.1 to 15.2 15.2 to 21.3 21.3 to 27.4 12,1 2627 Aug. 15, 1963 8.4 15.2 22,5 27.9 11.8 14,4 to 21.38 21.3 to 27.4 10,7 27.4 to 29.8 to to to to 15.2 22.5 27.9 30.0 Ambient 25.4 20.4 28.2 Radius* of particle 5,T.P. cutoff size (stage 1), u 6.20 0.16 1.98 0,954 6,18 0.12 23.4 22,3 23.2 43.1 5.55 2.14 0.793 0.646 0.16 0.18 0.12 0.12 24.4 22.6 32.3 5.72 2.21 1.18 0.16 0.20 0.12 14.6 14.9 19.8 56.4 3.37 1.33 0.700 0.844 0.16 0.20 0.12 0.14 22.7 27.4 to 29.6 to to to to , Volume, 31.4 0.351 0.464 0.12 0.12 *The sampler consists of a two-stage impactor with backup filter. The radius of the particle cutoff size for stage 2 for all flights was 0.02 u, Cutoff sizes are based ona 50% collection efficiency and a particle density of 2 g/cm’ at midaltitude for the sampling interval, Table 2—IMPACTOR-— FILTER COLLECTION DATES RELATIVE TO ANNOUNCED NUCLEAR TESTS* Approximate age of fresh-debris Collection Date of most recent nuclear test component (At), days Mar, 16, 1962 Sept, 25, 1962 May 16, 1963 Nov. 4, 1961t Within test seriest Dec. 25, 1962T 132 Fresh 145 date Aug. 15, 1963 Dec. 25, 1962T 236 *Only announced atmospheric nuclear tests’ with fission. yields greater than about 1 Mt have been considered. tConducted by U.S.S.R. at Novaya Zemlya (75°N 55°E). {The U.S.S.R. conducted about six tests in the megaton range in September 1962 prior to the collection date. Most recent test date for the U. S. Pacific tests (2°N 157°W) prior to the collection date was July 11, 1962. the test preceding our collection was conducted by the U.S.S.R. Our collection of September 1962 is expected to contain primarily a mixture of fresh nuclear debris from the U. 8. Operation Dominic Series and the U.S.8.R. 1962 series. We have assumedthat there is a negligibly small contribution of radioactivity to our samples from Plowshare cratering experiments and surface detonations at the Nevada Test Site during 1962. Data for total beta and total gamma activity on the counting date and for individual radionuclide concentrations on the flight date for 1962 and 1963 collections are presented in Tables 3 and 4, respectively.