products formed per KT of fission yield, plus 1.1 x 10° curies of beta-

active products, for a total of 4.1 x 10° curies of fission product
activity.

The average effective gamma ray energy in a fission product

field is about 0.7 Mev, so that if 1 million curies of mixed fission
products are spread uniformly over a one square mile plane surface, the
gamma radiation intensity measured 3 feet above that surface would be

about 4 r/hr.
The specific yields of radioactive materials have been studied in
%

a variety of ways.

The Hunter-Ballou studies?!

.

on slow neutron fission,

and Coryell-Sugarman compilation2/ ean be used to obtain percentage

values.

Zinc-72 is the atom of lowest mass and gadolynium-160 the

greatest of those found to result from fission.

Figure 1 indicates the

variation of fission yield with mass number, with fission yield exe
pressed as a per cent, for y> uv, and Pu’? ,

The total adds up to

200% since each fission gives two fission products. Fast fission of
uranium-238, plutonium-239, and uranium-235 results in approximately
the same fission yield values with the largest difference in the middle

zone where the value varies from 0.01% for uranium-235 to 0.05% for

uranium-238.

Thus, the various mixtures of fissionable material and

uranium-238 tamper material which may be present in a weapon have relatively little effect percentage-wise on the relative amounts of radioactive isotopes formed.

The first peak in Figure 1 includes strontium-

-89 and strontium-90 and the second peak contains iodine-131, which are

¥

—

Hunter-Ballou studies are an accurate measurement of the percentage

of radioisotopes obtained from a laboratory bombardment of uranium
and plutonium by slow neutrons. The results of the observations in
the laboratory are compared with the percentages of radioisotopes

found in fall-out particles and variations between the labcratory

and test percentages are an indication of fractionation. This
approach is considered the only accurate method possible to calculate percentage yield. ‘The Coryell-Sugarman studies provide similer information about the percentages of isotopes produced in the

laboratory from the bombardment of fissionable materials with fast
neutrons.
a

2/ Hunter, H.F., Ballou, N.E., Simultaneous Slow Neutron Fission of

U-235 Atoms, I. Individual and Total Rates of Decay of the Fission
s, USNRDL ADC-65, 1949.

3/ Coryell, C.D., Sugarman, N., Radiochemical Studies, The Fission Products, ine National Nuclear Energy Series, Book 2;

6

Part V, 1951.

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