of leaves. Strontium-90 reaches the human body by direct consumption of vegetation and of milk.from animals that have fed on the vegetation. Therelative importance of the various pathways depends on many factors, for example, the composition of the soil (calcium level) and the nature of plant cover. A heavy root mat will tend to trap fall-out strontium and delay its reaching the soil for dilution with soil calcium, while at the same time permitting absorption into the plant from the base of the stem. The agricultural management of crops and livestock, which includes the plowing depth, fertilizer practice, and type of feeding (barn or pasture) employed, is another factor to be considered. Also of great importance are dietary habits of the population and food technology. As anillus- cium. In all steps of the food chain from vegetation to human bone, calcium is preferentially utilized relative to strontium. Thus, it has beencal- culated that at equilibrium the strontium-calcium ratio in bones of young infants would be from 3 to 12% of that in vegetation, with values of 8 to 16% in the bones of persons over 6 months of age. Although milk is our primary source of calcium, the discrimination against strontium relative to calcium in passage from the feed of the cow to its milk tends to reduce the importance of milk as a source of strontium-90. While dairy products furnish some 80% of our dietary calcium, they may supply somewhat less than 40% of the total strontium-90 intake when steady-state conditions are established. Attention should also be given Tasie 1.—Comparison of Radioisotopes in Environmental Contamination collects in thyroid Barium-Ho 13 days like calcium, collects in bone = pe — of — 2 slow Samples for monitoring radicisotope levels... cece eee ee eee tent eenee Maxinum pertnissible radioisotope coneentrations, zue per litert,...... Radioisotopes in milk, zuc per liter$.. Comparative radiation dose to TUMTATIS, TAG... ce cece eens Strontium-s89 Cesium-137 Strontium-90 il days like ealeium, collects in bone 28 years like calcium, eolleets in hone slow alow co ~~, /\ relatively fast A y 7 vy, M-—— Man vegetation, inilk, amd thyroid vegetiution and milk 3,000 121 200, (KK) 42 7,000 Ag 80 6.4 150,000 57 <0.04 to thyroid in 7935 and 1956 <10% of strontitm-. approximately from approximately 0.2 to approximately 0.001 89 dose soil, vegetation, 30 years Uke potassium, collects in muscle \ sav a fast o— Removal rate from body............. Main pathways in food echain*....... 5 Metabolle behavior.............0...+5 Todine-131 8 days <A NN Physical half lHfe...........cecceercace milk dairy products, bone, and aquatic food 1 to 20% of stron- tiim-90 dose soil, yeretation, nulk dairy prod- ucts, bone, and aqiatie food (@.4 to skeleton over 70-yr. period from present yeretution, milk, dairy products, meat, ind whole body per year from present levels tests$ *A4 = atmosphere V = vegetation M = milk S = soil (' = eattle MP = ineat products. + Reconunended maximum permissible concentrations for specific Tadioisotopes in drinking water as derived from recommendations of National Committee on Radiation Proteetion and Meusurements. These concentrations and milk values are quoted by Public Health Service. t Levels found in United States from July, 1957, to July, 1958. § This estimation inchides recent analytical data and concepts of nonuniform stratospheric inventories developed at May, 1959, congressional subcommittee hearings. tration, in the processing of frozen vegetables, washing them prior to freezing will remove some of the surface contamination. If nuclear tests are stopped, the soil reservoir will become increasingly important: therefore, the time pattern of contamination has to be taken into account. Although food-chain considerations are extremely complex, certain gen- eralizations can be made. It is obvious that the pathways that require considerable time in passage to man (for example, via the soil) are of no significance for the short-lived radioisotopes,” iodine-131 and barium-140. It also appears that the present contamination of diets originates mainly from surface contamination rather than from the soil reservoir. The movement of strontium radioisotopes from soil to man is interrelated and, to some extent, governed by the simultaneous movement of cal- to contaminated water supplies as a possible source of strontium-90. In making estimations, the entire strontium-90 and calcium intake of the population must be considered. The soil reservoir probably will not be an important factor for cesium-137 because of the fixation of this element in the soil and its consequent unavailability to the plant. At the present time, about 60% of the cesium-137 content of the average diet is derived from dairy products, 25% from meat products, and the remainder from vegetables, cereals, and fruits. Radioisotope Levels The present levels of these radioisotopes in the biosphere (soil-plants-animal products—man) can be determined with reasonable accuracy by radiochemical analysis. For purposesof illustration, table

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