3} tea, it became evetrtifore difficult to extrapolate to body burden fromfood. The excretion rate of Sr?’ maybe expressed as the sum of two exponential functions for the Arst the transport of low levels of Sr’ and other prod- Sr’? is excreted eariy, with a biological half-life of environmental data alone ofthe internal radia- respond to those reported by Cowan! in a case of contamenated area. More reliable estimates of the Marshallese body extrapolating back to the one-day Sr8® bodvburden of the Marshallese.**, spectrometry and by radiochemical urinalysis. and Zn** are presented in Table 32. and also It is obvious that further data are required on ucts through the ecological cycle in this and other communities to make possible assessment from tion hazard to human beingsliving in a falloutburdens can be obtained by whole-body gamma Radiochemical Analysis of Urine Strontium-90. The urinary excretion levels of Sr°*° for the 5 years following exposure to fallout are shown tn Figure 55. The +- and 5-yearlevels were much higher, after the return of the Marshallese to Rongelap in July 1957, the mean being higher by a factor of 20 in March 1958 than in ee Nenean eer es ee oe ne cee ee en on ee ee eR Ree ee ee March 1957. 3 years following exposure. The major fraction of +0 davs. The smaller fraction is excreted witha half-life of 300 days. These excretion rates cor- accidental inhalation of Sr?’, and were used in The 1958 Rongelap body burdens of Sr®, Cs!*", figures for percent of equilibrium and equilibrium value, estimated by Woodward* from urinary excretion data. These values are subject to some uncertainties, since they are based on a number of assumptions; however, they can be checked by use of other methods. For example, the estimated body burden of Sr*° in March 1958 was 2 wuC/g Ca, based on the 24-hr Sr*® output in urine (1 hrer per 24 hr), and this appeared to be of the right order of magnitude compared with data from 10 ie ‘5 2 | bone analysis. Two bone samples of vertebra aad tleumvars from a deceased 35-year-old Rongelap Y geiap male at this time indicated a level of about 3.7 puCfreg 7 4 oO 4 Ca, which gives, upon application of the normali. te J zation factor of 2 from vertebra to average skele& F 1.0 58 7 1 the mean body burden of Sr*° for exposed Rongelap people in 1958 was estimated to be =2 muC, S o BO2b a O th~40 pay$ . « a |peTORN TORONGELAP R Eee AYP aye, ay . 300 800 900 1200 1500 1800 TIME IN DAYS ~ AFTER MARCH 1, 1954 ton,** an average skeletal value of 2 uuC/g. Thus : or about 9% of the estimated equilibrium value of 4 23 mpC.*° . . The estimated Sr** body burden increased from 2 mpC in 1958 to 6.0 mzeC in 1959, or 26% of the estimated equilibrium value. The 1959 Sr9° mean urinary value in the exposed Rongelap inhabitants was 6.3 upC/! or 10.5 puC/24-hr urine, based Figure 55. Urinary excretion of Sr”? in exposed Marshallese. Table 32 Estimation®® of Body Burden, in muC, of Rongelap Population From Urinary Excretion Levels, 1958 Cs'3? Sr”, Exposed Body burden . Equilibrated body burden Percent of equilibrium Daily intake cS Exposed 2 23 9 0.015** *3.7 Strontium units (SU) determined by bone biopsy. **15 SU assuming daily calcium intake = 1 g. 118560! “900 1300 69 2(?) Zn Control Exposed 1200 280 1600 75 330 85 Control 540 2.1-4.1 650 83

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