se 38 magnetic tape of a 704 computer. The task of “spectral stripping” was carried out on the computer with a FORTRAN program. In this operation the spectrum ofeach individualisotope is removed from the total spectrum obtained for the subject, which represents the combination of the contributions from ail the isotopes deposited in that subject. Spectra for each of the individual isotopes quantitated in this study were obtained with the use of an Alderson phantom (REMCAL). Solutions of known concentration of each radionuclide were placed in the phantom to approximatetheeffects of tissue absorption and scatter. The spectrum of the phantom for each of the isotopes was obtained under conditions of counting geometry identical 00.000 pr mn GAMMA RAY SPECTRA OF PLASTIC Mana FE Cs"? (0942 pe, 0.66 Mev! 5 J 10,000 ~ COUNTS 30 MINUTES /20 kev CHANNEL E \ 2n** (0.463 yc, 112 Mev) S : 54 4 4 | ‘000 SPECTRUM | | ~ L 100 NET Zn*3ec3"" | : EF | 4 K id gk"146 Mev) ' , 4 1 _e NET TOTAL, maocy | | SPECTRUM | NET C37 “| 5 | 7 SPECTRUM i. [- with that used in counting the subjects. By this technique it was possible to simulate quite closely with the phantom the multicomponentspectra of = 5 the Marshallese. A representative Marshallese .- IK 4 20 44 68 92 He ENERGY 140 164 188 Mev Figure 35. Gammaspectrum otthe calibration phantom containing Cs'*. Zn"’, and Kin the approximate range found in Marshallese subjects. The dotted lines indicate the results of spectral stripping of the higher energy photopeaks. spectrum obtained by adding K, Cs'**, and Zn" at average levels (as determined in the medical study of 1959) to the phantom is shown in Figure 55. The K, Cs'*", and Zn"? were distributed homogeneously throughout the phantom. while Co" was placedin theliver only. Analyses of the complex spectra were performed by subtracting the calibrated pulse-height spec- trum for each gamma emitter to be quantified. Although these spectra are obtained ideally trom a subject of identical build, an approximationis i ie ll a o TT Lay “ETERNAL B- US MALE, MEDICAL TEAM AGE 41) YRS-WT=: 77 Kg Zn*(98 myc) CPA IO 2 myc) 18 de LL 5878 O88 ie ENERGY (Mev) ~~ t ‘ / i | I k { co fem 38 “> wo sat _ K(AtI39.4g 682140.3g) o TUTTtrity 5 hide die de COUNTS /30 MINUTES/20 kev CHANNEL +A a 38 158 Lititil A-MARSHALLESE MALE AGE 45 YRS-WT=70 Kg Po tea th os17 ye) Yaduiu obtained with the use of the plastic phantom. Figure 56. Spectrum of typical Marshallese adult male compared with that of memberof the U.S, medical team. Computation was carried out by an IBM-704 computer. Starting with the highest energy photopeak. that of K'° (after correction for background and normalization of the K*° photopeak to that of the subject), the computer performs a channel-bychannel subtraction of the normalized K’*”spectrum. In a similar manner, the normalized spectra for Zn**, Co®, and Cs'** were subtracted from the total spectrum (see Figure 55). Individual 24-hr urine specimenswere collected and one pooled urine sample of 20 liters. The radiochemical procedure for the Sr*° analysis has been described previously.’ RESULTS A spectrum for an average Marshallese adult male, obtained in the 1961 study, is shown in Figure 56, with the spectrum of a memberofthe U.S. medical team of about the same body weight

Select target paragraph3