ee enTee Se eh Bn ae ilRaia ee Ke Ailiarate Be t-Cs'37 (9542 jac, 0.66 Mev) | 4 iw 0,000 L{_ <i = | = 4 a : — = , Zn? (0.443 pc, 112 Mev) /- = a 4 —4 | S | | > a 4 { =x ° “ | = “1000 f= 5 2 FEI oO :e L ~ L_ E NET T 65 cgi 2n°"+Cs SPECTRUM | [ = | 10G = 4 : 4 _ “= NET TOTA | | O an Alderson phantom (REMCAL). Solutions of known concentration of each radionuclide were placed in the phantom to approximate theeffects of tissue absorption and scatter. The spectrum of the phantom for each of the isotopes was obtained under conditions of counting geometry identical with that used in counting the subjects. By this techniqueit was possible to simulate quite closely with the phantom the multicomponentspectra of the Marshallese. A representative Marshallese spectrum obtained by adding K, Cs’*’, and Zn at average levels (as determined in the medical : Mev) >_| K**140gk",146 | z 5 titated in this study were obtained with the use of — SPECTRUM NET cs’? 7 o SPECTRUM io 20 44 68 q 92 116 ENERGY Mev 140 164 study of 1959) to the phantom is shown in Figure 55. The K, Cs'*", and Zn*° were distributed homo- 188 Figure 55. Gammaspectrum ofthe calibration phantom containing Cs'**, Zn’, and K*"in the approximate range found in Marshallese subjects. The dotted lines indicate the results of spectral stripping of the higher energy photopeaks. TOT A-MARSHALLESE MALE t COUNTS /30 MINUTES/20 kev CHANNEL TT AGE 45 YRS-WT=70 Kg [ iO A = = B- U.S MALE,MEDICAL TEAM AGE 41 YRS-WT-77Kq e Zt L ~ - —s - — F 2r°°(98 myc] 10° CAH 102 myc} K{A=139.4g a uh . \ cs712 5 myc) | “ss, 1? E- i \ t ot \ LS _ i ‘ } , 5 B=140.3g) 9 + 4 7 / \ i —_ -{ 4 ey f \ 8 t j 1 \, WAY * } by s---~- NLA ee a 4 / | 48 38 58 398 118 ENERGY {Mev) 78 4 138 oj} _. (158 _ eS ci tt = fot RESULTS __! Figure 56. Spectrumof typical Marshallese aduit male compared with that of memberof the U.S. medical team. ae) tota] spectrum (see Figure 55). Individual 24-hr urine specimens were collected and one pooled urine sample of 20 liters. The radiochemical procedure for the Sr*" analysis has been described previously.’ 4 4 fot subject), the computer performs a channel-bychannel subtraction of the normalized K"° spectrum. In a similar manner, the normalized spectra for Zn"’, Co*", and Cs'** were subtracted from the 4 7 | fey toi. dt ! geneously throughout the phantom, while Co*° wasplacedin theliver only. Analyses of the complex spectra were performed by subtracting the calibrated pulse-height spectrum for each gammaemitter to be quantified. Although these spectra are obtained ideally from a subject of identical build, an approximationis obtained with the use of the plastic phantom. Computation wascarried out by an IBM-704 computer. Starting with the highest energy photopeak, that of K*° (after correction for background and normalization of the K*" photopeak to thatof the A spectrum for an average Marshallese adult male, obtained in the 1961 study, is shown in Figure 56, with the spectrum of a memberofthe U.S. medical team of about the same bodyweight eeante en magnetic tape of a 704 computer. The task of “spectral stripping” was carried out on the computer with a FORTRAN program. In this operation the spectrum of each individualisotope is removed from the total spectrum obtained for the subject, which represents the combination of the contributions from all the isotopes deposited in that subject. Spectra for each of the individual isotopes quan- — Rtlettin a LETaeANN ple — cnn — > GAMMA RAY SPECTRA OF PLASTIC MANS ws eect lle e n cen Nn 100,000 & 2 an etme ot ence mee” Mla Naty 38