te radioactive material accounted \jor part of this activity was conline. Fig. 3 shows the percentage ticulate form at different depths two samples collected within the f particulate radioactivity in the ose slightly at 48 hours. However, 1m) and inside the thermocline -rose at an increasing rate during he percentage of radioactivity in xponential rate from a value of 48 hours. ig edges of the particulate radio- i, and those of the soluble-colloidal ie 28—48 hours the leading edges ity in the mixed layer descended ie mixed layer during the entire vpproximately 2.5m per hour. oactivity in the particulate form in the mixed layer. During the ity moved down at least 200 m, or approximately 10 m per hour. This mayreflect the separation of the particulate matter into a heavier fraction, which was observed at 6 and 28 hours as deeper concentrations of radioactive particles and which sank below the mixed laver ahead of the remaining particulate activity. During the last 20 hours the heavier particles descended rapidly through the thermocline. The failure of the radioactive contamination to become evenly distributed throughout the mixed layer might be attributed to the short duration of the observations on the movement of the radioactive material in the water, although this is probably not the case. In the area of the test site, at least, the combination of the effect of gravity on the particulate activity plus the rapid movement of the surface waters (above 25 m depth) tends to cause stratification in the mixed layer of sufficient magnitude to overcome, in part, homogeneous mixingin this layer. The ability of phytoplankton to concentrate radioactive materials and to remain near the surface probably adds to the tendency towards stratification in the mixed layer. Homogeneous dispersion of the radioactive contamination throughout the mixed layer may occur after sufficient time has elapsed, as indicated in the WALTON SURVEY (JUNE 11-21, 1956) 4 DAYS TO 23 DAYS ASTER CONTAMINATION ‘ «MARSH SURVEY { SEPT. I-20, 1956) 6 WEEKS AFTER ENO OF TEST SERIES -21, 1956) IR CONTAMINATION ~-+-~ COLLET? Survey (auG. 3-14, 1958} AT END OF TEST SERIES nee SILVERSTEIN SURVEY (SEPT 2-13,1954) a WEEKS AFTER ENO OF TEST SERIES -20,, 1956) TEST SERIES a-14, 1958} TES RANGE OF UPPER ECGE QF THERMOCLINE sEPT. 3-13, 1958) OF TEST SERIES 19,000 . 9,000 + 8,000 E 7,000 > - uw = = a =t [tg 6,000 r 5,000 4,000 }-— 3,000 2,000 F. teu VALUES MULTIPLY 7000+ * 300 ES 400 _ soluble plus colloidal fraction in all cing 1956 and 1958 between the EniGuam 0 2550 100 180 200 250 300 ano DEPTH IN METRES Fig. 5 Total radioactivity in water samples from four oceanic surveys made during 1956 and 1958 between the Eniwetok Test Site and Guam § 113 “nf