48 F ri to Zn (1 12 Mev) a tet = > cr 3 L r { b F Nw = | 1000 s ° 5 Z = presence and concentration of other components or cs37 (0 66 Mev) 100E Cc F E 5 3 b b L 1 i : 1 \ zn*hs cs” \ NET UN IVO-—"7' CONTRIBUTION | 40 ts"? SPECTRUM | Kv) 46Mev) \ i ‘ NET TOTAL BODY + SPECTRUM L t . 24 in i 48 1 ‘2 i “a 36 120 L ENERGY (Mev) laa 4 ab i . i6a—~=C«*' 2 Figure 53. Gamma spectrum of phantom illustrating graphical stripping of K*°, Zn**, and Cs'*’ from total spectrum. one isotope to the photopeakof the otherisotopes of lower energy is very small. In orderto carry outthis stripping method,itis necessary to have calibrated pulse-height distribution spectra for each gamma emitter encountered. Further, these spectra must ideally be obtained from a subject of the same size and bodybuild. To obtain these spectral data, known amounts of Cs'** and Zn® were administered to subjects at BNL, and their spectra were obtained. Laterin the study, a plastic phantom (REMAB-Alderson) wasobtained andusedfor calibration (Figure 54). of the spectrum. This procedure was further complicated in this study by severalfactors. In thefield study the subjects were measured with a 5-in. Nal (T1) crystal. The calibration was originally carried out in the field with a Presdwood phantom, but when the Alderson plastic phantom later becameavailable it was foundto give a better approximation of the spectrum for each isotope, and therefore most of the calibration was repeated with it at BNL. However, the geometry in the field situation was rather difficult to duplicate exactly. Also, counting the subjects for 5 to 10 min was sufficient toestimate accurately the levels of Cs**’ and Zn® but not the K*° body concentration and trace amounts of otherfission products in the presenceofthe relatively large amounts of Cs'*’ and Zn**, Thelack of a statistically significant number of counts to measure K*° accurately is evident from the poorly defined K*° photopeakof the subject as compared oo 10,000 patton Spectra were also obtained from the phantom with known amounts of KCl, Cs'*’, and Zn®. From these spectra, an average spectrum for each isotope was obtained. The pulse-height distribution spectrum of one of the Marshallese subjects is compared with the spectrum obtained with the plastic phantom containing the same concentrations of K, Cs'*", and Zn® in nearly identical counting geometry in Figure 52. In this way it was possible to simulate the multicomponentspectra of the Marshallese by use of the phantom. Since it is not possible to measure a photopeak until the contributions of other peaks of higher energy and their Compton continua have been subtracted out, and since the presence of small amounts of unknown radionuclidesis not always ence of very small amounts ofother fission products. However, when all the major components have been stripped out, the presence of any remaining photopeak should serve to identify the Figure 54. Calibration phantom in standard counting position in BNL whole-body counter. os obvious in the presenceof large concentrations of other radionuclides, it is possible to miss the pres-

Select target paragraph3