Measuring

transuranics

in the air
For further information contact
Joe Kordas (422-6809).

The U.S. Department of Energy’s Office of Health and Environ-

mental Research is interested in improving the sensitivity and

response time of air exhaust monitoring systems at nuclearfacilities.
At LLNL, we have developed and fielded a very sensitive alpha
measurement system for determining the concentration of trans-

uranics and other long-lived alpha emitters in the air. In tests at the
Rockwell Hanford Operation’s facilities in Richland, Washington,

the system proved to be at least 100 times more sensitive than
presently available monitors. —

Large quantities of long-lived

alpha-emitting substances (such as

radium, thorium, uranium,
plutonium, americium, and
curium) are or will be handled at
nuclear laboratories, fuel fabrication plants, chemical processing
facilities, and future waste
repositories. Online monitoring instruments play a critical role in
evaluating and minimizing the
release of such substances through
exhaust stacks to the environment.

The monitoring
environment

An online alpha detection
system for stack effluent must be
able to withstand high moisture
and acidity and yet detect small
quantities of long-lived alpha emitters in the presence of a much
larger, natural alpha background
consisting of the daughters of
radon-222 and -220. Radon-222
and -220 are gases, but their

daughters are charged and thusattach themselves readily to particles
ment System (TAMS), recently
that are collected with long-lived
developed at LLNL (Fig. 1), is
alpha emitter samples. Figure 2
capable of measuring extremely
shows an alpha eneray spectrum of
small quantities of transuranics
this daughter background taken at
(elements that have an atomic
atmospheric pressure. The colored
number greater than 92) or other area indicates where the peak
long-lived alpha emitters in short
caused by long-lived plutoniumtime periods. TAMS will makeit
239 would fall if it were present.
possible to assess both normal and Under normal conditions, at locaaccidental releases rapidly.
. tions 1 metre above the ground,
radon-222 and -220 concentrations range from 0.04 to 0.4 pCi
perlitre (20 to 200 times the 40-h
maximum permissible occupational
concentration for plutonium-239
A Transuranic Aerosol Measure- ~

in air).

14

Select target paragraph3