60

conversion factor for each sample (density) was then approximated by interpolation, assuming that the actual conversion factor varied linearly with

density between the range of factors determined in the 1.17 and 1.35 g/cc
standards.

The error that could result due to a nonadherence to the linear dependence
assumption described above was estimted by considering the case where density
changes give rise to logaritnmic rather than linear changes in the correction
factor.

The maximum error that could result from a logarithmic instead of the

assuved linear dependence was estimated by finding the difference in the value
cf the two correction factors which occurred at the extremes of sample density
encountered in this work (0.6 and 1.6 g/cc).

The difference in correction

fectors thus determined, using the two different correction factors, was 7.3%
fcr the sample geometry and density limit which yielded the highest error when
counting 60 KeV gamma rays.

For radionuclide concentrations which were deter-~

rined by using higher energy gamma-rays, and for the majority of samptes which

were not at the extreme limts of densities, the error which could arise due to
this uncertainty is smaller than 7.3%.
The abundance of each y-ray observed for a radionuclide (Table 11) was
used to calculate the concentration of the radionuclide present.

Where more

than one radiation from one nuclide was observed, the reported value is that
cerived by weighting the concentrations determined from each gamma peak observed by its associated relative counting error, and a weighted mean concentration and error was determined (Stevenson, 1966).

The error term associated

with the counting of individual energy gamma-rays are 2 S.D. errors based on
propagated counting statistics.

The concentrations of all the isotopes measured by y-spectrometry in this
work are corrected for decay to the date of the collection shown in Tables 3
and 4,

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