99

of the refractory radionuclides on the Ca0-Ca(0H)o - CaCO, particle matrix
which was deposited here.

Despite the source of 234y and 238) measured in

these sediments, a slight 235y enrichment is indicated for the 8-10 cm sediment section by the low 238))235, ratio measured.

If either of the second two possibilities given are responsible for the
observed uranium concentration differences with depth in the core, the inereased concentrations of

226

Ra and

210

Pb, which appear to be similarly

enriched in upper sections of the core, can be explained by the same process
responsible for the elevated uranium concentrations.

Similarly, since it is

difficult to envision an artificial pathway for the production of 2269,, the
first possibility noted above is not consistent with increased concentrations
of

226

Ra in the sediment.

The third case above is no different than the

primary fractionation of radionuclides first described by Freiling (1962)
except that naturally occurring, rather than bomb produced, radionuclides
are involved.
Station B~2 Sediment Core

The distribution of 210p, (21954) and

226

Ra concentrations measured in

the Station B-2 sediment core are shown in Figure 24. The concentrations of
2105, in the surface sediment of the core is about four times higher than that
which can be supported in situ by 2264 decay, again indicating an external
source for the 210 Pb measured.

The 2195, concentrations in the upper 12 cm of

the core decrease at about the same rate as do the 24) a and 23942406, concen-

trations.

Although the rate of decrease in lower layers is not well defined,

th e 21951, 7226p, ratio decreases to 1 at a depth somewhere in the 11 to 22 cm
region of the core.

Such concentration profiles for

210

Ph are typical of

marine sediments accumulating 2105, from natural sources (Schell, 1974b).
The concentrations of

226

Ra measured in the 2-4, 8-10 and 14-16 cm sections of

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