isotopes in appreciable amounts. Detailed studies were undertaken to establish with certainty the identity of the isotopes and to determine their contribution to the total activity in the Rongelap soil. MATERIALS SND Mz THODS A 1.68-gram portion of soil ash, equivalent to 18.1 grams of dry soil, taken from the top inch in a bird nesting area at Kabelle Island on July 18, 1957, was dissolved in 0.2 N HCl and passed through an ion-exchange column to separate the radioisotopes present sample. in the (The method used was described in detail by Lowman, Palumbo, and South). 14 For this experiment a cationic resin (Dowex 50*) of 50- 100 mesh and column size of 0.942 cm2 x 61 cm was used. The sample and the eluting agents were passed through the column at a flow rate of one ml/min. A summary of the volumes used and the radioisotopes eluted is given in Table 1. Aliquots of the fractions collected were counted for beta and gamma activity, and those fractions with significant amounts of gamma radioactivity were analyzed in a single-channel, 50-position, automatic-advance, gamma spectrometer with a 2-inch, well-type sodium iodide crystal. M7 * Available from Dow Chemical Co., Midland, Michigan Tak Te ‘4 pet ot. yt boy wer ve, Nr Seger 1e5 ¢ey fi : Bet So * ct . epey, ” Mea ae s . ¥ », ae te EG eigen . we tj . 2 we 7 a

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