fy,

156

the absorbed dose delivered to the stomach in
i hour ig small.

The absorbed dose in the top

portion of the small intestine is the same as
that to the stomach, but decreases during the

4 hours there due to the 60 percent uptakeinto
the bloodstream. ‘The absorbed dose to the
large intestine is much greater than that to the

small intestine because the radioactive material
speuds 8 hours in the upper and 18 hours in
the lower large intestine compared with only
4 hours in the small intestine. Also, the mass
of material in (he upper or lower large intestine

is aboutone-eighth of (hat in the small intestine

ONy=150 gg, Mu (35 g, Mg=1100 g,
Mytomsen*= 250g). In the case of Ra”the 6-hour

daughter, Ac”, makes a large contribution to
the dase. Therise in the dese in the small intestine is accentuated by the fact that the
effective energy of Ac? is 80 times that of the
parent, Ra?*, and there is only 20 percent
absorption from the small intestine into the

blood,

ct

THE SHORTER-TERM BIOLOGICAL HAZARDS OF A FALLOUT FIELD

The slow rise in the absorbed dose in

the upper and lower large intestines in the case

of SP°+¥", and Ra**-+-Ac is the result
of the growth of the 61-hour Y®*, and 6-hour
Ac™® respectively. In the case of the 17.5minute Pr, the absorbed dose is delivered

mostly to the stomach. The dose to the large
intestine is negligible because Pr' passes
through17 radioactive half-lives in the stomach
and small intestine.
The foregoing tables of MPC values maybe
useful in dealing with hazards associated with
the fallout material from the testing of nuclear
weapons as well as the contaminationresulting

from a laboratory spill or accident.

However,

manyof the radionuclides of great interest that

comprise fallout during the early periods follow-

ing the detonation of an atomic weapon were
not included in these tables. There are many

factors that determine the type of fallout
material from the detonation of a nuclear

weapon, e. g., height of burst, distance from

ground zero, typo of weapon, weapon yield,
meteorological conditions, ete. Likewise it has
been found that there maybe factors (physical,

chemical, and biological) which tend to frac-

tionate and concentrate certain of the radio-

INTERNAL DOBE FROM SHORT-LIVED RADIONUCLIDES

157

nuclides. For example, at the first Bikini
underwater test I made a numberof surveys on
the target ships and nearbyislands of the 8/y
dose rate rrtio and found it to range from 1 to
several hundred. This high 6/y dose rate ratio
was, in part, a consequence of the fact that on
the. average there are about twice as many

radiation. In any case, the record should
speak for itsclf- namely, the damage to man
and animals (cattle, horses, deer, etc) that

unless measurements have been made of the
absorbed dose from # and soft + radiation.
Having called attention to the many factors

exposure to hard gamma radiation but from

have risked setting up Table III which lists
the more important U-fission radionuclides that.

disintegration of the U-fission mixture, and
most of the beta particles have a range of less
than a meter in air whereas a large fraction of
the gamma photons have a range in air of
manymeters, i. e., the fraction of photons with
an absorption coefficient d that travel a distance

cautious not to overlook the seriousness of

fractionation.

beta particles as gamma rays emitted per

has been observed from the fallout material
from nucleartests to date has resulted not from
exposure to beta radiation. In assessing the
hazard from fallout, therefore, one must be

exposure to beta radiation, and one should not
rely on a theoretical estimate of the isotopic
distribution or one should not reach final
conclusions regarding the radiation hazard

greater than x is given approximately by the

tain circumstances this fractionation maybe of

considerable importance because overexposure
to beta radiation can lead to serious erythema,
burns, ulcera, and even death. Yet the most

commonly used field survey equipment is
designed to measure the absorbed dose from
relatively hard gammaradiation and may give
little or no response to beta radiation. Following the test of a thermonuclear weapon by the

United States in the South Pacific in 1954, the

more serious cases of radiation damage among
the natives and operating personnel from the

United States: resulting from contact with the

fallout’ materials were the consequence of
exposure to beta radiations. It is sometimes
stated that beta exposureis oflittle importance
compared to the gamma dose from fallout

material and that one would have to be partly
naked or lie prone on the ground before the
beta exposure should be a matter of concern.*

T do not agree with this point of view and dare
say some among the Marshallese, the Japanese
fishormen, and the Americans who received

painful and disfiguring beta burns as a cansequence of exposure to fallout material in the
“South Pacifie would not be inclined to underestimate the seriousness of exposure to beta
“Thereader is referred 1o the final summary ofthis Conference by Dr.

K.P. Cronkite.

would be presentas a function of time following

the detonation of a weapon if there were no

The radionuclides are listed in

order of decreasing availability (assuming no
selective deposition or separation of the radio-

elements) for 5 time intervals—1 hour to 1 day,
1 day to 1 week, 1 week to 1 month, 1 monthto

Tante IIT.--AVAILABILITY OF U-FISSION RADIONUCLIDES

equation (1—e>*). In addition, many common materials such as tar, resin, rusi, paint,

metals, etc., seemed to retain selectively certain
of the beta-emitting radionuclides. Under cer-

which may change the isotopic distribution, I

(Listed in order of decreasing yield)
Thour to 1 dey

Radionuclide

t week to 1 month

T day to 1 week

1 monthto I yeur

1 year to 70 years

Yield

Radionuclide

Yield

Rudionuclide

Yield

Radionuelide

559
519
458
454]
451

Mo... 8s.
Cel... 2]
Nb? 1.)
DR...
pit.

360
360
250]
241
937)

Lal__ re
Bato
~w--f
Pri@ __
Cettt__.
DH.

444
427
423
414
387
376
363
351)
314
294
250
233
222
206
164
163
161]

Zr"...
Tet?,
Bat®_..
Lave.
-|
Palo... -]
Pri®. 2...)
Y%_Srt._
Pmt.
Nd¥7___
Rho
[5_.
Celt,
Zr.
¥"__
¥e_.
Sri.
~

229
228
160
128
122
U1
Hid
9G
92
77
70
48
40
39
37
37
35

Nd¥7_
Zr%6___
Y%_.
Sree_.
Mom,
Rue.
Rhee,
132 |
.
Tet?___ wees
Obes, e weee
Cet4...
Pret.
Cela...
Pm'@..

337
293
284)
216
160
128
127

Nb... 2...)
Zr... 22)
Yo.
Sriv_.
Cem,
Ces...
Prt _.

586
483
374
311
284
271
271

Sr. 12... }
Ye
Cet? .
-.
Bat7_
Pm
Cems.
Pris,

480
430
406
406
215
214
214

96
93)
87
79

Lave. _
Baio __
Pm¥?.. _...
Nd...

150 Rhtes_
135 Zr%__
44 ya .
et

27
14
9
4

28

Rhis_

72
71
70
67
61

Rh 2.
Pris. oo...

31
7

126

37
34
2

Ru... 2.)

32

122
109
102

4h]
28
14}

12)

Vield

Rus _
Rnie__
Pri___

ym le
Ruts,
.
Sr

-|
-

¥8_.
Cit
a
Bat?__..

197
189
154

34
22

22
13

13
10
10

Radionuetide

Smit
Nb®.
Ruts,

Yield

44
31
27

Select target paragraph3