ed by the ar. Com‘der of 14 n and soil from the ; made by chosen by maximizing the percentage variation for which the model could account. The percentage variation accounted for is defined by > (M,—ayXnO.9, — 03gn)” V=1—" ; = [10] ' missing ‘monthly where 4, isthe observed milk level in the n month and Jf is the average observed milk level for 7 months. The parameter values for the optimal model are shown in table 3. Note that the «’s differ from region to region, reflecting the differing relative emphasis on the soil level and deposition rate factors. The percentage variations accounted for are smaller in stations wherethereis less variability in the milk levels. From inspecting the varia- ie overall . constant *e plotted example, is missing g overall le. Then, suries per e for the rates will 959, The uld occur rlons are ted rates. on those er greatly h they get alf-times. ation was bility of the milk levels during the barn-fed period when one would expect them to be essentially constant, we can see that one could hardly hope to account for more than 50 percent of the variation in some of the stations. The results from the best model for each station are shown graphically in figure 4, where solid and dotted lines represent observed and expected (calcuJated) values respectively. The average predicted values are based on the assumption that the deposition rates will be about what. they were in 1959. Discussion Percent Variation wecounted for The sharp peak which sometimes appears in October, November, or December, and is not: fitted well by the theoreti- cal line might be a result of using feed from an >, (A4,—M)? n=l 1 of the sampling variation. It is interesting to note that the estimates for the parameters in areas of similar environmental conditions are close to one another. This is particularly reflected in the pasture halfresidence time 71,2. The areas of low rainfall, Sacramento and Salt Lake City, have a longer residence time than New York City and Cincinati, probably because of a much slower washout. Also, the «’s are very similar in the similar areas. Since the deposition rates contain a large element of uncertainty, some of the minor peaks are missed occasionally. In periods of low dep- osition, one would not expect to predict fluctua- tions of minor magnitude. The predicted line remains essentially constant during the months of barn feeding so that the deviations of the observed values during this period measure the Vol. 77, No. 12, December 1962 early spring harvest. This factor might well account for the fall peak sometimes observed and should be investigated. It seems reason- able on the basis of figure 4, however, to assume that the model is capable of predicting large fluctuations if the correct deposition input is known. Obviously, we have considered quite a range of deposition inputs. The future milk values will probably be a little less than the predicted line shown as “expected.” Estimates in May 1962 place the expected deposition from 0 to 20 percent less than in 1959. The milk levels of the five stations were averaged to arrive at national average observed and expected milk levels. Figure 5 showsthe observed milk levels along with the levels calculated by Knapp and the model presented here. He predicts an average of 15 micromicrocuries of strontium 90 per liter for 1962, whereas our model predicts an average of 11 micromicrocuries of strontium 90 per liter. However, if the fallout deposition should be twice what is expected at every station, our model predicts an average value of 15 micromicrocuries per liter in the U.S. milk supply for 1962. Then, on the basis of fallout deposition predictions and transport assumptions, it becomes possible to predict milk levels for any given future time period in segments of the country where the required measurements are available. This leads to a muchbetter esti- mate of the average yearly bone marrow dose in any region. Summary A mathematical model has been developed for the purpose of predicting strontium 90 concentrations in milk. It is the successor of several other models designed to predict the activity of radionuclides in milk. A relatively large yield of strontium 90 is deposited on the surface of the earth as a result of nuclear weapons tests. This radionuclide then finds its way through the food chain to human beings. Milk is one of the most important contributors to the total dietary intake. 1061

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