levels present (compare with soil data in Table 2). Additional work is under
way to determine the extent to which this finding is related to physical and
chemical differences in source material and to edaphic characteristics.

The

activity levels for these radionuclides in fruit pods were from one-tenth to
one-hundredth of the levels found in the forage tissue. The CR values for Pu
in soybean leaf and stem tissues ranged from 10-" to 10-3, and the fruit pod

values ranged from 107© to 10°*.

Fox Am, the CR values ranged from 1073 to

107! for leaf and stem tissue and 10°

to 107% for fruit pods.

It should be understood that the CR vaiue is a ratio of the vegetation to soil

activity level which expresses the relative uptake of a radionuclide through
the plant root system.
It should not be misconstrued to be an index representing contamination hazards even though it may give an indication, for a
given contamination condition, of the relative proportion of that contaminant
which might be expected to be incorporated in vegetation through the plant

root system.

We believe that »rerhaps the most important finding from these experiments
pertains to the greater uptake of 24 1am through plant roots in proportion to
the uptake of 2385 240p, demonstrated by these experiments.
The magnitude of
this differential uptake can be ascertained by comparing the Pu/Am ratios for
vegetation (Tables 3, 4, and 5) with the Pu/Am ratios for the soils on which

the plants were grown (Tables 1 and 2). In spite of the erratic data for
barley (Table 3), the Pu/Am ratios for plant tissues were, in many cases, much
less than the average Pu/Am ratio of 6.74 for Area 13 soil. Data for alfalfa
(Table 4) conclusively showed greater uptake of 24lam over 239°240py uptake by
a factor of at least ten for the unamended soil.
In those cases where the
acidulation amendment had markedly enhanced 239°240py uptake, this effect was

still around a factor of 5. Even higher factors indicating preferential
uptake of 24!am through roots are evident from the soybean data in Table 5.

We believe that this differential uptake characteristic for Am probably contributes to the slightly lower Pu/Am ratios often encountered for vegetation
samples collected in the aged fallout areas (Romney et al., 1974, 1975) compared
to Pu/Am ratios for the soils.
The impact of this finding for 24lam uptake

assumes greater importance when coupled with the fact that this radionuclide

is an ingrowth product of the source material in the aged fallout areas (Fowler
and Essington, 1974).
About 50 years of time still must elapse before the
ingrowth of this radionuclide will peak out.
It appears, therefore, that
potential problems from Am are equally as important, if not of greater concern,
as the aged plutonium source material in these fallout areas.

FUTURE PLANS

As the result of experimental findings, work on the soil amendments has been

discontinued, except for chelating agents.

The acidulation effects of sulfur

have no practical value other than to raise the question of whether or not
these transuranic radionuclides might be more available to plants in the event
of future contamination problems at sites involving acidic soils.

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