'-80 per cent of the fall-out dosevith Gustafson’s results?” during 159, when more than 90 per cent ose rate at a location at Argonne found to be derived from these mon? obtained similar results at Britain at about the same time. Laboratory has therefore develcurate determination of environ© partial dose-rate contributions and fall-out emitters utilizing chamber and y-spectrometric These techniques the field. umptions as to tho distributions 3 various radioisotopes and on procedures for interpreting the than 200 sites in the United open-field y-dose rates from y over a wide range from place ‘enerally falling between 5 and here high natural levels (up to ed, high thorium and potassium ily responsible. The relatively yw range of the observed dose- 9 uranium series are interesting ier study, and are probably uranium-238 and radium-226 and the migration of free ayers of the soils, 1962 and 1963 it was observed the environment had elevated isurable amount at every locaQ per cent or more in the total ® common over open ground, ere observed during the spring umn 1963 readings were lower, 7ith those a yearearlier in the iern New England. A decline 16 New York City area sites in sast four months of quite large 4l background-levels. These hose of Burch e¢ al." in Engand April 1963, who recorded ‘ somewhat elevated readings ast-November 1962 and then it. above normal y-background untained except for the effect pril 1963. There is also rough data’, which seem to indicate ission product dose rate at a Laboratory from 2 ur./h to 962 and July 1963 and then a “> . declme to 3 yur./h by October 1963. With the signing of the Test Ban Treaty, it is expected that the decline in fall-out y-dose rates observed in late 1963 will continue, but at a much slower rate as the long-lived '*Ru-!%*Rh and ¥7Cs replace "Zr—*Nb as the dominant contributors. Any assessment of the significance of the fall-out data presented here in terms of population oxposure-levels should take into account the relevance of open-field dose- rate determinations to such considerations and the degree to which the years 1962 and 1963 can be treated as typical for conditions of substantial weapons testing. If we reduce our open-field fall-out measuroments bya factor of two to account for the offect of structural shielding as suggested by Spiers®, and by another factor of two to correct for weathering processes not taken into account in our measurements, it would appear that an increase of the order of 10 per cent in total oxternal environmental radiation exposure has been experienced by the popula- tion of the United States during this two-year period. If this is reasonable, it seems probable that, diring and shortly after periods of significant nucloar weapons testing, the exposure of the general population to environmental y-radiation from deposited fall-out is not noghgiblo m comparison with that duc to the natural radiation environment. 1 0’Brien, K., Lowder, W. M., and Solon, L. R., Rad, Nes., 9, 216 (1958). 4 Solon, L, R., Lowder, W. M,, Shambon, A., and Blatz, H., Science, 131, 903 (1960). 1 Shambon, A.. Lowder, W. M., and Condon, W. 4, Health aid Safety Leth. Rep, HASL-108 (1963), ‘Sievert, R. M., Arkiv. Pysik.. 16, 347 (1059). * Spiers, F. W., Nature, 184, 1680 (1959). *Vennart, J., Vature, 185, 722 (1960). ? Gustafson, P. ¥., Marinelli, L. D., and Brar, 8. 8., Seltence, 127, 1240 (1958), * Gustafson, P. F., Radiology, 75, 282 (1960). * Peirson, D. H., and Salmon, L., Nature, 184, 1678 (1959). © Collins, W. R., jun., Welford, G. A., and Morse, R. 8., Scienec, 134, 980 (1961). "Collins, W. R., jun., U.S, Atomic Energy Comm. Rep. TID-7632, 271 (1961), 88 Gustafson, P. F., and Brar, 8. S., Health Phis., 9, 629 (1063). ' Gustafson, P. F., and Brar, S. &., in The Natural Radiation Enrironment, edit. by Adams, J. A. S., and Lowder, W. M. (Univ. Chicago Press, 1964). ™ Burch, P. BR. J., Duggleby, J. C., and Spiers, F. W., in The Natural Radiation Environment, edit. by Adains, J. A. S., and Lowder, W. M. (Univ. Chicago Press, 1964). % Lowder, W. M., Condon, W. J., and Beck, H. I.., in The Natural Radiation Environment, edit, by Adams, J. A. 5., and Lowder, W. M. (Univ. Chicago Press, 1964). 1 oe A. B., U.K, Atomie Energy Authority Rep. AERE-R-4137 2a 17 Kartashov, N. P., Atomnaya Energiya, 10, No. 5, 531 (1961), transL, Sov. J. dt. Fn.,10, No. 5, 526 (1962). In English 1“ Wollenberg, H. A.. and Smith, A. R., in THe Natural Radiation Envirenment, edit. by Adams, J. A. 3., and Lowder, W. M. (Univ. Chicago Press, 1964). 1® Gustafson, P. F., Argonne Nat. Lab. Rep. AN£5967, 156 (1959). 20 Friend, J. P. (ed.), Defense At. Support Agency Rep. DASA-1300, Part 3, Chap. 3 (1961). 13

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