ae te ath samples was taken so that the variation of isotopic concentrations with depth might later be investigated. A, Instrument ation Spectrometer System The HASL spectrometer system consists of a 4 in. x 4 in. NaI detector with preamplifier and high voltage battery pack. a 400 channel multichannel analyzer and parallel printer. a DC~AC converter and a 12 volt storage battery. The calibration of the detector is described in detail in previous HASL reports”’’*. In brief, the exposure rate due to a particular isotope in the ground is inferred from the number of counts under a spectrum total absorption peak characteristic of that isotope using calibration factors determined from a combination of laboratory experiments and theoretical caicuiations. The prominent tctal absorption peaks observed in all the field spectra (see Figure 2 for a typical field spectrum) were at 1.17 and 1.33 Mev {°°co), .10 Mev (** Eu), .44 MeV (*"®sb), and .662 Mev (“*°’cs}. These isotopes appeared to be responsible for almost all of the total expcsure rate at the spectrometer locations. Individual exposure rates for *$7cas, °°co and -*"Sb were inferred for each field location. The “°° Bu exposure rate was assumed to be of minor importance due to its very low source energy. For those lccations where the ionization chamber was nct used or the other total exposure data were inconsistent, the spectrometric data were analyzed to obtain total exposure directiy’. Except for the two Eneu locations, all spectra were taken in ten minute runs. During this time there was no appreciable gain shift due to temperature changes. In almost all cases we were able to obtain excellent field spectra with only minor equipment maifunctions even though the equipment had to be carried by hand through heavy brush, loaded and unloaded into small boats in fairly rough surf, and operated and stored in ambient temperatures of approximately 85 95°F and relative humidities of 70 - 80%. Ionization Chamber - Our high pressure ionization chamber has a 5.6 liter sensitive volume and is filled to a pressure of about 700 psi with pure argon gas*., The chamber wall is eo "3 PoP, wie po