-12-

both dust and sea spray so that the total mass obtained by integrating the
volume distribution and multiplying by a density factor would not be expected
to agree with the dry, residual mass loading measured by HV andCIP.
The relatively good agreement obtained between the different measurement
systems indicated in Tables 1, 2, and 3 gives us the confidence to draw conclusions about the significance of resuspension for enhanced inhalation exposure
in this worst case example.
If the total plutonium activity (pCi g-l) is obtained
by integration of the curves of Figure 1; we find that there is a significant
change in the aerosol plutonium activity relative to the plutonium activity of
the surface soil. Let us define an enhancement factor (EF)
as follows:
.
~F

= total

aerosol

activity

(pCi g-l)

.

soil activity (pCi g-])
Upon investigation of the enhancement factors, we find that the values apparently
were less than one under normal conditions (Table 4) probably because of
selective resuspension of non-radioactive particles whichserved
to dilute the
plutonium activity.
There is no evidence how this occurred.
Marten
surmises
ratio values should be greater than one, but gives no evidence (8). The ratio
of organic particles to calcareous soil particles remained about constant (10%)
as determined by X-ray fluorescence on the PD filters exposed at this site during
the same period. Me know from previous studies that one component of organic
matter, plant leaves, had a ratio of 10-3 plutonium concentration relative to
soil and could serve to dilute the inorganic aerosol. )
-.
TABLE 4.

Enhancement factors for plutonium activity of aerosols on Bikini
Island (HV data).

Soil
Activity
(pCi q-l)

Aerosol
. .
~;;;v;:$

5/6-8

15.3

47.5

3.10

Stabilized bare soil

5/10-11

15.3

14.7

0.96

Stabilized bare soil

5/12-16

15.3

10.5

0.69

Coconut grove

5/8-16

8.01

Road with traffic

5/8-16

4.10

Site
Disturbed-bare

Date
soil

3.29
10.3

Enhancement
Factor
::_:

0.41
2.5

Under dusty conditions, EF values exceed one such as in the cases of the
disturbed bare soil (3.1) and the road with ”traffic (2.5). So_there.are. two.
.djfferent factors producing increased plutonium aerosol concentrations
(aCi m-3~
ciyr.i.ng-unusual
resuspension.
T~e...aer~~ol_dust“concentration
increases,
but also
.__..
the plutonium activity.increases.
For e~ample, averaged over 10 HV instruments’
._..,.---.,
..... - . ..--4- -...- .
.
.

/

, ..-.<
.
L ..

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