248 SESSION I DISCUSSION kilometers of air, I was wondering whether or not the natural aerosol concentrations in these large volumes would be sufficient to add anything appreciable to the weight of the debris and tend to produce this effect. ~ BENSON: I don’t think so. A high-energy thermonuclear device is a fairly heavy weapon, and, at these fairly high altitudes, the natural aerosol is small. The contribution of dust raised from the groundis insignificant. Therefore the total mass engulfed at high altitudes would be rather small. I think the main reason, however, for this peculiarity les in the fact that we are talking about large particles, in the neighborhood of 5 to 15u. With respect to the radiochemical analysis of these particles, one of the facts we did not bring out in the paper was that the volatile constituents had yields of less than the independent fission yield. Values of barium were found, for example, which were 0.003 of what they should have been in relation to what the zirconium was. This implies that at the temperatures at which particles of this type are formed (roughly the boiling point of aluminum oxide, which is rather high) elements like rubidium and barium are volatile. The first member of the *Zr fission chain is rubidium. think the effect is caused by a volatilization of the early precursors within the fission- product chains. Although we think of the refractory fission products as being distributed evenly throughout the mass of the weapon, this does not appear to be true. When we are talking about large particles, the fission products are all potentially being reduced rather than being enriched or evenly distributed throughout the volatilized mass. FOOTE: I would like to know the approximate costof Dr. Nielsen’s spectrometer. , NIELSEN: It cost us than $50,000 today. about $70,000. It can be obtained for less BENSON: While we are talking about costs, I would like to ask Mr. Foote how he gets the $0.15 per analysis that he mentioned. FOOTE: That is the total cost of readin and readout. MILLER(C, E., Jr.): I would like to point out that we have in progress a program on the fractionation of fission products as part of the Nuclear Safety Program at Oak Ridge National Laboratory. It is sponsored by the AEC’s Division of Reactor Development and Tech- nology rather than the Division of Biology and Medicine andis, therefore, not being reported here. However, I do feel that the work is pertinent to the fallout program. We are interested in amounts of fission products contained in transported materials in a reactor accident and in any information «> can extract concerning the mecha-

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