In addition to the tuna from the Japanese fishery, sixteen
yellowfin tuna, believed to be from a single school, were caught

off Bikini Atoll in the Marshall Islands in September 1969.
Liver samples,

not obtainable from the Japanese-caught fish,

and

light muscle and dark muscle from these fish were analyzed for
gamma-emitting radionuclides,

iron-55 and stable iron.

The samples were counted for 900 minutes each with 3-inch x
3-inch Nat(Tl)

analyzers,

crystals used in conjunction with 256-channel

Spectrum reduction was done by Schonfeld's

method of least squares,

(1965)

and all values were corrected for decay

to the date of collection.
Iron-55 was separated and purified by a combination of

solvent extraction and electrodeposition techniques
Beasley,

1967).

Recoveries generally exceeded 90%.

(Palmer and
Counting was

done by X-ray spectroscopy with a proportional counter used in
conjunction with a multichannel analyzer.

Some duplicate samples

were analyzed by different persons using different methods,

ard

the results were in close agreement.
RESULYS

The values for

55

.
tuna had a wide range.

Fe,

The ranges for dark muscle were

to 1600 pci/g dry weight;
oo.

aclivity,

.
toes
tos
.
stable iron and specific activity in

.

0.02 to 8.6 nCci

iron, 49 to 500 ppm;
35

Fe/mg Te.

55

Fe,

and specific

3.3

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