é 3 Table 2. Contribution of pasture to iodinc* 131 burden of cattle. Millimicrocuries . of I" per gram Animal number of fissue (fresh weight) 3 5 13 100 101 102 Barn-fed cattle 0.0092 0.012 0.012 0.013 Thyroid Doses _ It is of interest to estimate the radia- 0.013 0.08 tion dose received by the thyroid glands of the humanandcattle populations during the period of this study. The level of iodine-131 in an individual at any given time represents a balance between the Avg: 0.012 Pasture-fed cattle 16 0.042 18 Ce ‘0,039 , fall-out is deposited on the forage and the time the dairy product is consumed. This may be an important factor and should be looked at more carefully under situations where milk from grazing animals is consumed within a matter of days after secretion. intake, perhaps from several tests, and Avg. 0.041 the biological and physical removalrates, _This makes it difficult to calculate inSpat Ae having thethyroid levels shown in Fig. 1 should have been about 0.2 millimicrocurie per 100 milliliters at the 1955 peak and averaged about 0.02 for the whole’ period. These values are higher than those found, probably because dairy cows usually consume older feed than do the cattle reported in this article. The data in this article do not permit estimations of the contribution of iodine-13! carried in milk, although the low milk levels found and the fact that the levels in younger age groups werenotsignificantly higher would indicate this route to have been of minor importance. The contribution of milk is, of course, decreased by the physical decay between the time the Table 3. Examples of spread in iodine-131 levels in human and cattle thyroids. All continental samples except from Nevadasouthern Utah area. May 1955 Human No. of samples Percentage of samples with Less than 0.0008 mpc/g Betweeen 0.0008 and 0.01 mpc/g More than 0.01 muc/g Cattle No. of samples * Percentage of samples with Less than 0.001 muc/g Between 0.001 and 0.1 mpc/g More than 0.1 myc/g August 1956 101 60 29 62 60 11 35 3 20 ° . 22 10 0 40 86 50 14 . finity dosages in the usual way (8). By integration of the area under the curves in Fig. | and estimation that 1 millimicrocurie of iodine-131 per gram of tissue delivers about 0.012 rep per day, it is calculated that the tetal dose from the iodine-131 beta rays, delivered over the 23-month period to the thyroid gland, was about 3 rep for cattle and 0.01 rep for man. In considering thyroid dosages, it is necessary to take into.account the contribution of short-lived isotopes of iodine. This situation has been analyzed by Dunning (8), who shows that, up to 10 hours after detonation, the short-lived radioiodines may contribute’ about 4 times the iodine-131 dose and by 2 days about equally, but that after 10 days the contribution of the short-lived activities becomes negligible. It is not possible to correct the over-all dose of iodine-131 for the contribution of the short-lived activities, but in any event the total dose could not have been greater than 4 times the average dose from iodine-131 (4x 0.01 rep) for man and was probably muchless. There seemsto be little question that the levels of radioiodine introduced into the biological cycles by weapons tests during 1955 and 1956 are far below those that are expected to produce any observable effects. This can best be demonstrated by comparison of levels found with the official maximum permissible values and with findings on the lowest levels of radiation or of iodine-131 that could possibly have produced detectable changes. Such a comparison follows. 1) Average peak level observed in man, 0.005 millimicrocurie per gram. 2) Maximum permissible level in man for continuous exposure (9), 15 milli- microcurie per gram. 3) Estimated peak level in milk, less than 0.01 millimicrocurie per 100 milliliters, 4) Maximum permissible concentration in water for continuous exposure (9), 3 millimicrocuries per 100 milliliters. 5) Estimated average dose to human thyroid from radioiodine during the period January 1955 to December 1956, less than 0.04 rep. 6) External dose to neck area in infants and children that has been suggested as cause of later thyroid malignancy (/0), 200 to 725 roentgens. 7) Dose to thyroids of sheep on daily intake of iodine-131 at which no damage was observed (11), 936 roentgens (3 rocntgens per week for 6 years). 8) Dose to thyroid of sheep on daily intake of iodine-131 at which minor physiological change occurred (11), 3000 to 5000 roentgens (over 242 years). References and Notes 1, L. Van Middlesworth, Nucleonics 12, No. 9, wo a * R. L. Gunther and H. B. Jones, U.S. Atomic 56 (1954). Energy Commission Document UCRL-2689 and addendum (1954). 3. M. R. White and E. L. Dobson, U.S. Atomic Energy Commission Document UCRL-3355 (1956). a . L. Van Middlesworth, Science 123, 982 (1956). This work was performed at the Medical Di- vision, Oak Ridge Institute of Nuclear Studies, Qak Ridge, Tenn. under contract with the U.S. Atomic Energy Commission. 6. Cattle thyroids and milk sampies were supplied through R. Miller, Omaha, Nebr., and with the cooperation of the Army Veterinary Corps, Office of the Surgeon General, and the Department of Defense. Human thyroids were received from Nicholas J. Chetta, Orleans Par- ish, New Orleans, La.; John H. Childers, University of Texas; T. H. Cochran, University of Utah; James R. Dawson, Jr., University of Minnesota; David Freiman, Beth Isract Hospital, Boston, Mass.; Nathan B. Friedman, Cedars of Lebanon Hospigal, Los Angeles, Calif.; Marvin Kuschner, Bellevue Hospital Center, New York, N.Y.; Kenneth P. McConnell, Veterans Administration Hospital, Louisville, Ky.; Hans Popper, Cook County Hospital, Chicago, Il.; Leopold Reiner, Beth Israel Hospital, Boston, Mass.; Vinton D. Sneeden, Emanuel Hospital, Portland, Ore.; and Walker B. Sorrell, Tulane University. The cooperation of these persons is gratefully acknowledged—it is emphasized that the succes: of this program depended largely on the procurement and prompt handling of uncontaminated samples. 7. C. L. Comar and R. H. Wasserman, Progr. in Nuclear Energy Ser. VI, Biol. Sei. 1, 153 (1956) . 8 G. M. Dunning, Nucleonics 14, No. 2, 38 (1956). ‘ 9. U.S. National Committee on Radiation Protection, “Maximum permissible amounts of radioisotopes in the human body and maximum permissible concentrations in air and water.” Natl. Bur. Standards (U.S.) Handbook 52 (Government Printing Office, Washington, D.C., 1953). 10. D. E. Clark, J. Am. Med. Assoc. 159, 1007 (1955). \l. L. K. Bustad e¢ al., U.S. Atomic Energy Commission Document HW-38757 (1955).

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