ADDENDUM

Quantitation and Char id ication:
fel)

Minimum Detectable
10

FCi/liter at

Range of
Lo-

10

Vu

in

tevel

far Urine

(LASI. procedure):

y47 coufidenee Limits
urine

trom Bikini

Islands

(EML procedure):

FCi/tteer

*EML, has ceased

its Pu analysis operations since

Plutonium concentration

in Rongelap/Utirlk Islands:

teeth samples (initial

data):
Ronyelap

1854167

£Ci/gm

Utirik

2074198 £Ci/gm

tooth weight between 1 and 2 gms
Definitely detectable using the BNL procedure.
Note:

Bikini/Rongelap or Utirik ratio for Pu in urine is comparable

however,

Pu in soil
2)

Assumptions

(EML data)

Bikini/Rongelap Pu in soil is at least 4X and Bikini/Utirik

that

is

20X.

have to be made insolying for the Pu body burden from

excretion data
a.
b.

3)

ICRP LOA excret iguymodel holds for Marshallese
Distribution of
Pu in man model (see attached)

‘the average error of 25% expressed in I.
LASL accuracy for
precision is

239

is applicable

Rationale 1(b) needs to be corrected.

.
.
g
Pu determination in urine is 100Z

!102Z

chemical recovery ranges 41 - 46%
24 hour urine sample for reference adult man - 1.4 1/day
Some samples ure as low as 340 ml/day whlch amounts to 764% error.
An
average of 890 ml/day results in 36% error.
The error then averages
46% and can be as high as 86% as long as the chemical recovery factor
is known accurately aud no other systemic error come

contro]

to

play.

A

urine program to screen non-24 hour samples should decrease

the erroc considerably.

9009553

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