Table 1.
Location
Bikini Atoll
Bikini Lagoon
Aomen-Yurochi Islet
Aomen-Yurochi Islet
Bokonejien Islet
Bokonejien Islet
Bokonejien Islet
NamuIslet
Eniwetok Atoll
Japian Islet
FElugelab Islet
Belle Islet
Bete Islet
Rongelap Atoll
Kabelle Islet
Kabelle Islet
Kabelle Islet
Palmyra Island

LEAD-210 IN SELECTED ATOLL SAMPLES
Sample

CollecCollecatop
tion
tion
(d/m/g/ dry
date depth(cm)
wt)

Sediment,
Soil
Soil
Crater sediment
Crater sediment
Crater sediment
Soil

1949
1967
1967
1964
1964
1967
1964

0-12
0-1
+ 0-3
Q-12
G-12
0-12
13-16

6440-10
2-74 0-05
2-0 + 0-05
4:5 +0-07
4-1+0-05
3-34 0-04
0-5 + 0-02

Soil
Crater sediment
Soil
Soil

1952
1964
1954
1954

0-1
Q-12
0-3
0-3

2440-05
3-8 + 0-06
0-7 40-03
0-440-02

Soil
Soil
Soil
Soil

1961
1961
1961
1962

0-0-6
06-12
0-8
0-8

4340-08
1440-04
2-7 40-06
0-6 + 0 03

0-1-2:2 d/m **Ra/g dry coral, while concentrations in
samples from depths of 60 m were 2-3 d/m ***Ra/g dry
coral.
The greater concentrations at depth result from ingrowth of 2?*Ra from the parent radionuclide, *U. In
addition the concentration of #1°Pb in rainwater is approximately 5 d/m/l. (refs. 10 and 11). and therefore a reasonable
estimate of the naturally occurring *}°Pb concentration
in coraline soils is several d/m/g drysoil.
My results, Table 1, show concentrations of 24Pb that

do not exceed those expected to occur naturally. The
=6Ra content of crater sediments and deep core sainples
should be about the same, as they are. Soils would be
expected to contain concentrations of #?*Ra of 0-1-2-3
d/m/g dry soil, depending on the depth sampled, the degree
of equilibrium between 22*Ra and its parent, ?3*U, and the

amount of particulate matter associated with the fallout;
the latter is a mixture of coral from various depths and
hence variable in 22*Ra content. Thomas'? reported the
207Bi content of the crater sediment collected at Bokonejien
Islet in 1967 as 200 d/m/g dry sediment. By contrast,
the 7°Pb content of the same sample is 3-3 d/m/g dry.
If?°Pb had been produced in significant amounts during
the testing programme, the concentrations in the crater
sediments would be much greater than they are.
It seems unhkely that the US tests of 1958-59 or 1961-62
contributed significantly to the #°Pb content of the
atmosphere.
Production by USSR tests cannot be
discounted due to differences in structural materials in
and around the device, but the absence of any reported
2077Bi in worldwide fallout associated with these tests
casts some doubt on this possibility.
I thank Professor E. E. Held for selecting the samples
and for helpful discussions. Ehis work was performed
under contract between the US Atomic Energy Coinmission and the University of Washington.
T. M. BeasLey

Select target paragraph3