the activity found in the 0- to 5-cm samples.

Analysis of selected

The
samples for cesium-137 indicated a similar vertical distribution.
distrisource
cesium-137 data did not indicate the Rocky Flats oriented

bution reflected by the plutonium-239 data.

The results (activity per unit area) for the 0- to l-cm and O- to 5-cm
sampling techniques exhibit about the same relative uncertainty, although
the trend of the data indicates that the results for the 0- to I-cm
technique are somewhat more variable than the results for the O- to
5-cm technique.
The average coefficients of variation are 42 and 30
percent, respectively.

INTRODUCTION

Investigators have applied numerous sampling techniques for plutonium in

soil (reviewed by Bernhardt, 1976).

The techniques are generally tailored

to match the investigator's program objectives; e.g., primarily inventory
or hazard assessment, which in most cases is for airborne resuspension.

The Nevada Applied Ecology Group (NAEG) techniques (Fowler et al., 1976)

and those described by the Nuclear
Guide 4.5 (NRC, 1974) are oriented
emphasis is to account for most of
is stipulated as including the top

1974).

Regulatory Commission Regulatory
towards inventory determination.
The
the plutonium; and a surface sample
5 cm of soil (Bernhardt, 1976; NRC,

Since most of the plutonium is usually on the surface, the distribution
of plutonium is fairly uniform at 5 cm, and small errors in the sampling
depth will have a limited impact on both the mass of material sampled
and total plutonium sampled.
An error of plus or minus 1 cm will only
affect the mass of material by about 20 percent for a O- to l-cm sample.
The phenomenon of resuspension has been reviewed by Oksza~Chocimowski

(in press), Lem et al.

(1977), and Anspaugh et al.

(1975).

Sampling for

resuspension assessment must include the plutonium concentration in the
surface layer of soil and the size distribution of the plutonium and
associated soil aggregates.
Particle size, which is important but
difficult to realistically determine, has been studied by Bernhardt,

1976; Johnson et al., 1976; Little et al., 1973; Tamura, 1976, 1977.

The depth involved in resuspension mechanics is not clearly known, but
is dependent upon an array of soil and climatological factors and is
generally believed to be within the surface 1 cm.
The proposed Environmental Protection Agency (EPA) guidance for trans-~
uranics in the environment specifies soil samples be related to the top
l cm, and the soil fraction less than 2 mm (10-mesh sieve) in diameter

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