then done once more, to confirm that the intended particle had indeed
Photomicrographs were prepared of each particle for the
been mounted.

record, but also to accompany the mounts for recognition by analysts.

OBSERVATIONS AND RESULTS

When the alpha emitter is contained in a small particle of a few millimicrons diameter or less, the tracks in the nuclear emulsion are radially
oriented and appear to have emanated from a well-defined central point
or very small area.
However, when the alpha emitter is randomly distributed over the surface or throughout the volume of the particle, the
orientation of the tracks is more random, although the general appearance
of a star is maintained.
Therefore, if one observes the track star
generated by a large particle, or in a small particle attached to or
incorporated in the large particle, one can determine the manner in
which the alpha-emitter is incorporated into the observed particle.
The

application of these inferences to our observations on the isolated

particles yields the result that, with the exception of the particles
isolated from samples 16910 and 16911 and a few particles from samples
17153 and 17154, the plutonium is present in small particles attached to
large ones, presumably soil.
Generally, there was little difference between the particles from the
two locations near a given detonation point.
The exception was the pair
of samples 16910 and 16911.
The particles in 16910 contained a large
amount of plutonium compared to the particles in samples from other
Slides, and were easily recognized and isolated.
Only one such particle
was isolated from sample 16911.
A number of other particles with plutonium were initially located on the slides, but these particles could not
be isolated.
They may have been very small particles attached to large
particles, becoming separated from the host particles during manipulation, or they were very fragile and broke up when attempts were made to
isolate them.
Selected isolated particles are shown in Figure 2.
The results of our measurements are listed in Table 1.
The plutonium
concentrations in the particles have been calculated as though the
plutonium is distributed homogeneously throughout these particles.
This
fiction may have some validity if one wants to consider inhalation
hazards, but is useless if one wants to search for size dependence of
the concentration.
Such a search was made with the data from sample
16910 but no correlation was found, although the particles from this
sample were probably homogeneous.
It has been our experience, however,
that the variability of fission product and heavy element concentrations
in particles of any given size generally extends over one or more orders
of magnitude, so that 9 or 10 particles are not sufficient to establish
the presence or absence of a concentration-particle size with any degree
of confidence.

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