Tor UNCLASSIFIED SUMMARY The Problem This is the sixth in a series of reports devoted to the study of radioactive fallout particles originating from the detonations of nuclear weapons in various types of physical environment. The fallout particles described Lere were collected following a tower shot in Operation REDWING, at the Eniwetok Proving Grounds. As in previous fallout particle studies, the chemical composition and structure of the particles and the distribution of radioactivity within them was desired Findings The chemical compositions and structures of the particles were determined by studying thin sections of the particles under the petrographic microscope. The distribution of radioactivity within the particles was found by making radioautographs of the thin sections. Determinations of the chemical compositions were also made by X-ray diffraction analysis. Three types of radioactive fallout particles were found. The most common type was composed of radioactive dicalcium ferrite surrounding an inner core of altered calcium oxide. These particles were formed by the interaction of the iron dnd radioactive elements condensing in the cooling fireball with drops of melted calcium oxide derived from the coral sand which was carried up into the fireball by atmospheric turbulence. <A second type consisted wholly of radioactive iron oxide and was formed by the melting but incomplete vaporization of the steel. tower with subsequent oxidation of the liquid iron drops. The third type consisted of unmelted coral sand grains with small, black, radioactive spheres adhering to their surfaces. The small, black spheres were presumably formed by the direct condensation of vaporized material ITU mye er fe sane in the fireball. iii UNCLASSIFIED

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