Table 3—- ESTIMATED BURST DATES OF FALLOUT IN RAIN WATER Sampling Burst month (calculated Burst month (calculated month from average Sr®?/sr*® ratios) March September 1955 August 1955 November 1954 May June September 1955 October 1955 November 1951 February 1954 July February 1956 October 1954 April from average % Sr*) March 1954 to be realized. This is possibly due to enrichment of the Sr*® in fallout that would occur ina mixture of material from different test series. Therefore, the Sr**/Sr® ratio is the more sensitive indicator of the age of fallout and can be expected to yield a more valid estimation of relative freshness than the percent Sr. It is apparent, then, that July rainout is of more recent origin than any of the preceeding months. It has been hypothesized that fallout material that is entering the troposphere from the stratosphere has a selective entrance zone near the mid-latitude region. If the fallout material is old and originated from a high-yield device, it is probable that the debris is strato- spheric, and upon entrance into the troposphere it can be brought down in rainfall. It follows that there would be moreactivity in rain occurring near the mid-latitudes. Scatter diagramsof Sr®activity vs inches of rainfall for all months are plotted in Fig. 2. All values, regardless of location, are plotted, but stations below 40°N (an arbitrary limit) appear as black dots on the plots. It is visually apparent from the scatter of the points that 4 + J 3F- — oO ke z o = uu a = g3 ° ob _—f oO Oo e Oe e O ° o oO 4 —e e ° e 5 e o L 2 L L 4 6 | 8 {0 RAINFALL, IN. Fig. 2a— Regression of Sr™ in rain water on the amountof rainfall in March 1956. there is little correlation on an over-all basis. Considering a separation of the data at 40°N, there is better correlation found among southern stations. The specific activity (millicuries per square mile per inch) of rain water for these stations is generally lower than for northern sites for the duration of the sampling, and the specific activity at each site does not vary conSiderably from month to month. Since it has been possible to obtain better correlation by using the 40°N separation, this idea is expanded by considering even smaller areas. For this purpose four areas in different 347