Thus a large fractionation relative to fission products and radioactive carbon dioxide occurs.
Of course, there probably is some entrainmentof fission products on the surfaces of the falling

ice crystals by the Greenfield Brownian motion accretion mechanism. In fact, it is known that

about 1 per cent of megaton yield off-site fallout occurs in the early banded tropospheric man-

ner. This may be due to this entrainment and thus one would expect that the latitudinal distribu-

tions of early tropospheric fallout of both fission products and tritium water from megaton
yield bombsfired in the troposphere!! should be identical. No satisfactory data are now available to check this point. In the calculations in this paper the figure of 1 per cent for tropospheric contribution from megaton yields has been used.

3

CONCLUSION

The more recent data, particularly on bomb C"‘, when taken together with the earlier data

on bomb fission products and tritium, give us some confidence in our present understanding of
the fallout mechanism. All of these observations and considerations afford unprecedented op-

portunities for the study of meteorology and geophysics, particularly in an international cooperative effort such as the International Geophysical Year.

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® w Bb

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on

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1m

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