Y UNITED STATES ATOMIC ENERGY COMMISSION WASHINGTON 25, D.C. Decenber 26, 1956 Dr. H. V. Weiss Dr. 8. H Cohn Dr. W. H. Shipman Dr. J. K. Gong . ete 2Oan9 U. 3. Naval Radiological Defense Laboratory Ban Francisco 24, California Gentlemen: I enjoyed your report, USNRDL-455 on the Marshall Island contamina- tion from Castle. Your soil data need to be recalculated with the available caleium rather than total calcium as the basis for the Sunshine Units. Could you analyse these soils for available calcium so the total ecOlogical picture can be seen? These analyses be done by is isotopic dilution using a neutral solution of Ca’’ and being careful to use only the mininem amount of water so direct solution by bacterial action may net cecur. Also use plenty of soil, 2 or 3 pounds, if possible. If you wish, send send the samples here to me and I shall run then. I have done a number recently and the method works vel. (cf. Gmith and Blume, Boi Sci. 77, 9 (1958)). A soil from Canton Island has been analyzed but none from the Marshalls. ‘The Canton soil gave about 100 grams of exchangeable calaium per equare foot in the top 3 inches. This is as you see only a small part of the total caleium so the Sunshine Units in your Table 3.2 should be miltiplied by large factors. This wild bring them into agreement with the levels found in the herbage. Very sincerely yours, W. FP. Libby CC: Dr. Ponpkins Dr. Dunning ir. Eisenbud WMP

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