8

ny
ch

where

corrected
t between
true beta
thickness

counting rate observed with thickness
the sample and the sensitive volume
counting rate at zero thickness
of material between the source

it

3

and sensitive volume

mass absorption coefficient expressed in

em* /mg

-o

At

ln.

nt

Me A t

(32)

Ned a + counting rate at thickness t #A +
The best straight line was drawn through the experimental

points and the slope(m) was calculated accordingly. This method is

applicable for any energy or group of energies as long as the first

part of the absorption curve is a straight line on a seml-log plot.
Jt can be seen from the examples given in Appendix A that this is the

case ana, therefore,the aforementioned determination of FP, was used.

6. Self absorption corrections for the samples in question
were considered negligible, since the weight per unit area was kept

in general between 5 and 10 mg/cm®. According to Coryell and
Sugarman,a radioactive sample which has a weight per unit area of 5

to 10 mg/em? and has an energy greater than 0.4 Mev requires no self=

absorption correction._3/ Furthermore, according to Hunter and Ballou,

the nuclides with maximum
more than 1 per cent each
approximately 10 per cent
time the measurements for
at H plus 200 hr.

energies below this value which contribute
to the gross fission activity constitute
of the total activity of the sample at the
this report were made, 1.8. approximtely

Therefore, the error entailad by the assumption

of a negligible correction should be 10 per cent or less.

The

practice of ignoring this correction has been further justified by

comparison of the defined geometry mthod with fow=pi counting

techniques.9/ In these comparisons the experimental error ranged from
3 to 7 per cento

7.

The sample beta activity (A,) was treated by the above

corrections to obtain the sample activity (Aq) in disintegrations per

arinute «

Ay =

*p
FE pe

(33)

A table of correction factors as well as examples of
various correction determinations and the activities A, of the samples
at the time of counting are given in Appendix A.

The above method has been used to determine the disintegra-

tion rate of known mixtures of nuclides with excellent results.10/

Its use in the determination of the disintegration rate for a mixed
fission prcducts sample is believed to result in measurements within
10 per cent of the actual rate. It is true that secondary particles

(e.g. internal conversion electrons) will be detected as primary beta

perticles.

However, the error in disintegration rate due to this

36

Select target paragraph3