- second, 4- to determine the distribution of these seven gamma- emitting radionuclides in many tissues from each of the 11 whole tuna; and third, to determine the presence of iron-55 (Fe>>) in the tissue samples from the whole tuna with the greatest gamma radioactivity. The six fallout radionuclides above were selected, based upon past experience, in the samples. as the nuclides most likely to be present Cerium-141 (cet, and ce 44 also might be expected to be present, but because of the difficulty of obtaining reliable estimates of small quantities of low-energy Mev), gamma-emitting nuclides by gamma-spectrum analysis, (< 0.2 cel! and cel44 were not included in the list of nuclides that were determined routinely. If the gamma spectrum had suggested the presence of significant quantities of cerium or other radionuclides, additional analyses would have been made. The gamma nuclides were measured in a detector system with four pi geometry. The detector consisted of an eight-inch well and a three-inch solid sodium iodide crystal. In practice, a sample is placed on the three~inch solid crystal which is raised into the three-inch well of the large crystal, thereby com- pletely surrounding the sample with at least 2-1/2 inches of crystal. The counting efficiency of this system was about ten times greater than the efficiency of the system with.the single,

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