Te The sparsity of stations end the variability of the data neure it impracticable to draw an instantancous pieture of the world-vide distribution of Sr-90. However, it is possible to make a rough estimate of the average concentration and distribution of debris in the stratosphere over an extended period of the order of six months. Figure 6 shows the averase concentration of debris in the stratosphere as a function of altitude and latitude for two six-month periods, Januery - June, 1957, and January-June, 1958. The data at each sampling altitude and station were averaged over the period and corrected for the filter efficiencies given in Table 2. It is evident that the sixteen data points, each based on a mean of only a few observations with large variability cannot serve to define the stratospheric Sr-90 content of the world. distribution can be extracted. tHowever, some information as to the A series of isolines showing what is felt to be the most probable distribution based on the available observations are also shown, although there are admittedly many other logical patterns which may be drawn. A comparison of the two cross-sections shows that between the first half of 1957 and the first half of 1958, there appeared to be a general decrease in the Intensity of the gradients observed, principally due to a decrease in the enncentration of Sr-90 at the two northernmost stations at 65,000 feet. Another evident change is the increase at all levels over the Canal Zone, possibly as a result of the British thermonuclear tests in the Christmas Island area which occurred in May, June, and November of 1957. These tests may @lso be responsible for the increases at 90,000 feet over Texas and Minnesota. NaS The patterns shown in Figure 6 may be integrated to estimate the total stratospheric burden of Sr-90. This computation gives the equivalent of 7.8 MI of fission products in 1957 and 5.5 MP in 1958. (A computation based on 0.25 filter efficiency factor at all altitudes gives 12 MP in 1957 and 8 Mr in 1958). These figures can be compared with estimates of the stratos- pheric content made by budgeting the debris. Table 1 shows that about 39 MI had been injected into the stratosphere as of the end of 1957. of this debris has been removed from the stratosphere. However, much Libby estimates the mean removal rate to be about 10% per year, Machta and List about 20% per year. These estimates would result in a stratospheric content of 20 to 24 Mr 8 Revue La ou Sob TONS OF TH ARCriyo> OF THE NATIONAL ACADEMY OF SCIENCES

Select target paragraph3