d in surface soil, where
relatively high contamination levels foun

those for BM
<100 mesh results tend to be considerably higher than
most
Second, the ratio of BM to <100 mesh is not, in
fractions.
Concerning Question
n.
cases, eonstant over all levels of contaminatio
ns from
2, the error in estimating inventory using Pu concentratio

o of concentra<100 mesh rather than BM aliquots depends on the rati
rions in these two soil fractions which (as noted above) is not
Probably a conservative
constant over all concentration levels.
the Pu data in
estimate of the average effect can be obtained from
These are surface samples from the second stratum of Area
Table 6.
13, a low-level stratum as compared to strata closer to GZ at that

0.5
site. For these data, the average ratio (sieved/BM) is 2.6 +
(X + S.E.) so that the estimated inventory would be elevated by a

factor of 2.6.

For strata nearer ground zero, one sees from Table 4

for soil samples in the top 0-2.5 or 2.5-5.0 cm in stratum 4 (the

highest activity stratum for the TTR sites) that the ratio can be
expected to be closer to 15 or 20.

Hence, the estimated inventories

for these high-activity strata would be similarly elevated.
Turning to Question 3 as to whether Pu concentrations on sieved

samples can somehow be corrected back to BM fraction or "field"
conditions,

the data in Table 8 is presented for consideration.

These are profile samples from the TIR (a subset of those in Table 4)

for which

239-240

Pu concentrations were obtained on BM, <100 mesh

and >100 mesh aliquots.

After the 10-gram BM fraction was removed

from the total BM sample, as much as possible of the remaining ballmilled soil was passed through a 100 mesh screen, and the weights of
the total <100 and >100 mesh fractions recorded.

A 239-2405, concen-

tration "corrected" to field conditions can be obtained by computing

8 = b(ata)t eGra)- tf

(1)

where the letters correspond to the labeled columns in Table 8; i.e.,
a= weight of <100 fraction, d = weight of >100 fraction, b = uncorrected Pu concentration in <100 fraction, e = uncorrected Pu concentration in the >100 fraction, c = Pu concentration of <100 mesh corrected
to field conditions, and f = Pu concentration of >100 mesh corrected
to field conditions.
Hence, g is a "weighted" average, where a/(atd)

~ proportion by weight of <100

mesh soil, and d/(atd) = proportion

151

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