DISTRIBUTION OF TRANSURANIC NUCLIDES IN SOILS:

A REVIEW

E. H. Essington and E. B. Fowler
Los Alamos Scientific Laboratory
Los Alamos, New Mexico

ABSTRACT

The literature is reviewed to ascertain the degree of movement and the
distribution patterns for transuranic and uranium nuclides

in soils.

Typical plutonium and uranium profiles are presented and an attempt is
made to identify unique characteristics causing deviation from an ideal
distribution pattern. By far most of the distribution observations are
with plutonium and little is reported for uranium and other transuranic
nuclides.

INTRODUCTION

In the past decade interest has been growing in the environmental

im-

pact of certain transuranic radioisotopes because of their potentially
hazardous nature to man. The potential for dispersion of these transuranics due to accidental release from components of the nuclear fuel
cycle, improper radioactive waste management, accidental or purposeful
nuclear weapon incidents, and further redistribution of existing global
fallout and specific loci of contamination is being studied. There
has been specific emphasis, during the past few years, on determining
the degree of vertical migration of certain transuranic radioisotopes
in soils,

both in the laboratory and under field conditions.

Further

investigation on the environmental fate of transuranic elements is
urgently needed in order to assess their long term distribution patterns.
This paper reviews past documentation on the vertical distribution of
transuranic nuclides and uranium in the terrestrial environment under

natural or near natural conditions.
Observations made thus far will
aid in predicting future redistribution rates and indicating where
additional evaluations are needed.

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