-408-

The first Marshall Island workshop was organized and hosted at LLL
in June 1977 to discuss long-range planning for the DOE Marshall Island
programs. An open exchange of information between al! program
participants provided a valuable overview of the radiological problems
presently being investigated and those remaining to be studied.
In early summer of 1978, we plan to participate in a Woods Hole
Oceanographic Institution (WHO!) cruise to the Marshall Island region.

Along with Dr. V.T. Bowen of WHO!, we will conduct a variety of
plutonium biogeochemical

16.

studies

in several

regions around the atolls.

TECHNICAL PROGRESS IN FY 1978:

We completed the publications listed in Sec. 13, and, with the
data generated by FY 1977, we began writing several other documents

describing the results of our Marshal!

Islands program.

in various stages of completion, include the following:
@

These reports,

Renewal Rates of Cactus Crater Water. We describe the use of
rhodamine dye to estimate the tidal flushing characteristics

of Cactus crater.

A simple model

is developed to explain the

water residence time as well as the fate of the crater water
and its dissolved constituents.
Cactus crater is being
considered as the disposal site for radioactive waste
accumulated during cleanup operations.
The results of this

study permit us to evaluate the impact and fate of any
radionuclides remobilized to solution in the groundwater after
the crater is filled.

@

Remobilization of Plutonium Radionuclides from Cactus Crater
Sediments at Enewetak Atoll.
Data related to the rate of
plutonium remobilization from sediments to the water are
provided.
The remobilized plutonium has solute-like behavior,
passing readily through 0.45-um nucleopore filters and dialysis

membranes, and can be traced in solution for considerable
distances along the reef.
@

Plutonium Concentrations in Reef Fish at Enewetak and Bikini

Atolls.

We compare concentrations

in mullet tissue samples

from different locations at both atolls. Plutonium available
to man from the aquatic environment should be most highly
concentrated in food organisms with the smallest number af
plutonium transfers between abiotic sources and man. Mullet
are inshore fish and in their adult stage feed on detritus
extracting organic matter from sediments. This species is an
excellenc indicator since the plutonium levels in mullet would

be expected to be highest among reef fish commonly caught.
Concentration factors, isotopic ratios in the tissues, and

other relationships between plutonium concentrations in fish
and in the environment are discussed. Concentrations in fish
at Bikini differ from those at Enewetak but the average

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