samples were analyzed

for

plutonium, calcium-45, strontium-89, ruthenium-103,

iodine-131, and barium-140.

The I-131 analyses of the pooled urine samples of the

servicemen and Marshallese provided the basis for thyroid dose estimates by Dr. Harris
and Jater researchers.

Dr. Harris judged that 1-131 analysis was the most accurate; it

also led to the highest doses to the servicemen (Reference 9).
The basic finding of the I-131 analysis of the pooled urine sample was the
determination that, for an average individual, the amount of I-131 excreted in urine
over a 24-hour period at the time of the urine sample collection (D+17 days) was 4.0
nanocuries. That resuit is used to determine the amount of I-131 intake.

The amount of a radionuclide excreted in a 24-hour urine sample is related to the

amount of the radionuclide initially intaken (that is, inhaled and/or ingested) by

A(t) =O.°¢€.°
Q°£, YQ) .F F,

(5)

where

A ft) =

the amount (uCi) of the radionuclide in a 24-hour urine sample taken
at time t,

Q) =

the amount (uCi) of the radionuclide intake,

f =

the fractional amount of the radionuclide intake that is transferred
to the blood,

Y(t) =

the ratio of the amount (uCi) of the radionuclide excreted with a 24hour period to the amount (uCi) of the radionuclide uptaken by the
blood, and

Fy =

the fraction of the total daily excretion that is present in the urine,

To apply this equation, not only must the time t of excretion relative to that of intake
be known, but also, for a radionuclide mixture, the time after detonation/release.

18

7b

In

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