NONTECHNICAL SUMMARY The Problem In order to predict the radiation hazards arising from fallout and devise protective countermeasures against them it is necessary to determine the characteristics of the fallout particles. Among the important characteristics needed is the relationship between two important individual aspects of fallout particles, size and radioactivity. Previous studies have considered the total radioactivity associated with particles grouped according to size ranges. However, this approach does not consider the variation of radioactivity with particles of different shape, shape being an indication of the differences in the manner radioactivity is incorporated in the particle. Also, the methods used in past studies for separating the particles into size ranges did not prevent the break-up of some particles, of which the fragments were regarded as being smaller particles. These two conditions caused misleading results in the final data in attempts to quantitatively describe & relationship between the size and radioactivity of fallout particles. The Findings In this investigation, the shape, size, and level of radioactivity were determined for individual fallout particles. A wide range of radioactivity intensities was associated with each of the size groups and sizeshape groups of particles. In the case of particles collected at one station in the field, a possibility was indicated that the radioactivity is normally distributed over a size-shape group. This set of data also indicate that regarding a relationship to particle shape, radioactivity varies approximately as the square of the diameter for irregular particles and as the 3.7 exponential power of the diameter for spheroidal particles. In the case of dendrite~like particles, the activity varies with a function exponentially greater than the irregular particle Punction. 4ii

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