Above 50 u the relationships were obscure. The gross decay did not vary at all with particle size at early times, and only slightly at later times. (U) In the fallout from Shots 1 and 3, Sr99 and pat4© showea greater (v) Shot 4 fallout samples, principally liquid, obtained from a (U) The base surge sampling program was unsuccessful. (vu) No information was obtained on variations of composition with tendency to concentrate in the liquid phase than the other fission products studied. project 2.5b intermiftent faliput collector, indicated that the relative concentrations of Sr°? and Bal increased with the time of collection. distance. (vu) The preliminary reports of this work appeared as ITR-918; a special report, CRLR 435, WT-928 - DECONTAMINATION AND PROTECTION. Operation CASTLE. Joseph C. Maloney, Ernest EH. August 1955. CONFIDENTIAL~RESTRICTED DATA (U) Dhein, and Manfred Morgenthau, Test panels, 4 ft sq, of 14 building materials were mounted on the weather surfaces of two remotely controlled ships and a stationary_ barge. ~~ - allout. All surfaces were contaminated significantly with tenacious Vertical surfaces facing upwind became equally or more highly contarinated than horizontal or pitched surfaces, probably due to wind currents impacting the tenacious contaminant onto surfaces normal to it. A sequence of hosing and vigorous scrubbing operations resulted in con- tamination reductions of 40% to 70%, but with reductions on most surfaces being less than 50%. Scrubbing was the most effective decontamination method. Under the conditions of this test, painting and joint sealing had little effect while the washdown countermeasure reduced the initial contazination over 90%. hm A ey In each case, the activity per unit weight of active particles Cel*4, below 50 » was found to decrease regularly with increasing size, but in a different manner for each nuclide, indicating radiochemical fractionation. 6 A sample of solid fallout from Shot 1 was separated into 14 parpicle-size fractions, which were analyzed for sr89, zr95, Mo99, Bal4O,

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