~10- amount of cross-contamination between the radioactive elements separated by a combination of the Dowex 50 cation- exchange method and the Dowex 1 chloride complexing tecmidque. The results of the radioisotopic separations are summa- rized in Tables 1 end 2. In these samples the predominant figsion-product radioisotopes were the relatively short- lived Zr95-nb?5 (65 a), Cel44-prl44 (285 4), and in one sample, RuLOE_ Ry] 6 (1 yr). The fission products accounted for 22 to 37 per cent of the total radioactivity in the three analyses from which cerium determinations were made. In the other two samples fission products contributed at least 5.7 per cent (stations 57,58,59) and 44 per cent (stations 13,14, 15) of the total radioactivity. gr90-y90 were not detected in the lon-exchange separations nor were they found in fuming nitric acid precipi- tations made on duplicate aliquots from both the five samples and their filtrates. Of the non-fission radioisotopes, Fe55, Cod’, Co>S and zn©5 contributed almost all of the activity. Although C0? was present at an average level of only about one per cent, it has the longest half life (5.3 yrs) of the reported non- fission radioisotopes and is therefore important. The variability, mentioned previously, between the retios of Co>’ to zn©5 also was evident between Co57 and Co0©°, and between Co°5? and Fe>>. In Figure 4a, the ratios of Co57/C06° in the five plankton samples are shown; also, these

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