- iz [F. 411042 Cot Cen ee Bee, vos a A COMPARISON BETWEEN SPRING 1959 FALLOUT AND STRATOSPHERIC AIR CONTENT 5tP4 Oatione! Academy of Sciences , U. &. Werther Bureau . s, on node Ett ASgm Commson ‘ Articles: Yursyamall 1960 ™ In a note by R. J. List in an earlier report (HASL77, pages 39+h3),-tt-— was noted that rainfall at Westwood, N. J. and Pittsburgh, Pennsylvania after my about January 1959 contained Sr-90 which was highly dominated by debris which dated from the Soviet tests in October 1958. [ a by Le Machta and N. Muirayama® Thay | Arghives/Comms.onGEM Taken literally, over 75% of the Sr-90 could be attributed to the date of October 18, 1958. A similar and more extensive analysis is made of the fission products collected by Project Ash Can in the stratosphere since November 1958. i In this ; case, several short lived isotopes were used to determine an apparent "age" and a fraction of October 18th Sr-90 (Soviet debris). sented in Table 1. Z These results are pre- The ratios of radioactivity at formation and the half-lives C of the radioisotopes were taken from (1) and are the same as were employed by i. Table 1 shows that the origin of the bulk of the stratospheric Sr-90 after . ee List for the fallout calculations. , November 1958 is more likely Hardtack or earlier than the October 1958 Soviet test series. Further, it shows that (except for the Ce-1¥4/Sr-90 results which will be discussed below), much less than 75% of the Sr-90 was attributable to October 1958. We shall first discuss some of the possible sources of error in comparing the apparent age and fraction of Sr-90 from October 1958 in fallout and stratospheric samples. We will then describe a meteorological interpretation result- ing from this difference. The computation of apparent age from a pair of fission product radio-~ L isotopes is subject to several sources of potential error. bee First, fractionation of the isotopes is known to take place. Thus, the [ assumed thermonuclear fission yield ratio for Cs-137/Sr-90 is usually exceeded by a significant factor in the stratospheric samples. | This departure from the [ ratio might also be due to erroneous estimates of fission yield of either radioisotope or due to differing efficiency of collection by the fallout or ro stratospheric sampling procedures. | .L- Japan Meteorological Agency assigned to the U. S. Weather Bureau, ~ isi . remee ME re a ~ fe CULLECTIONS Doe “yes Uy THES to AL AC ALE MY OF erteNceS | [ ,

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