RADIOACTIVE CONTAMINATION OF AREAS IN THE PACIFIC OCEAN FROM NUCLEAR TESTS CHAPTERIll Table 22—Summary of Gross Beta Activity in Water (NRDL)* Berta Activiry (8-/minfiter) Radiochemical Analyses SOURCES OF WATER [sLaND Ocean Lagoon Bide Cis! Ocean Bide Top NDA 12 290 6,300 260 23, 000 56 Well Bottom NDA 330 NDA tera Barrell NDA 1,350 16,000 28 430 Ex Tree Bole Soi! - d Profile — #4,000 14, 000 4 8,100 60 170 28 170 {. ” 38, 000 by AFL no radiostrontium was found. Tables 28 and 29 show the radiochemical analyses made by NRDLfor the February 1955 survey,2 and Tables 30, 31, 32, and 33 for the "Collections made about February 3, 1955. Date reported as of March 1, £055. February 1956 survey. Table 34 shows addi-~ tional analysis of soils from the February 1956 survey including data on exchangeable calcium. Tables 4, 5, 6, 13, 14, 19, 20, 23, and 35 show analyses by HASL. In terms of a potential biological hazard the Table 23—Results of Analyses Performed at HASL WATER Nowozn NuMBER} 43 390 7s 87 788 187 830 1003 1036 SaMPiiNe Location TYEE Rongelap......---.---.---| Well or eistern----....-.-.-Enisetok. Utirik. do. do. do. Ltklep. Lens. Well... do. Cistern. O-Dar ore 5 8-56 5 S& 5 856 8-56) 8-56) 8-86 d/m/l Torat Activity 2800432 sre djmfl Cit dimA % Sx 1% Cat? a strontium-00 activity is of most interest. Bich 3415 animals from Rongelap, Utirik, and Rongerik, 18:24:16 Nt Gejon_.... Enlactok.... 1008 Eniaetok. 1024 Bifo. 1081 Liktep...._... 1029 Utirik. *O-Date: Date af counting At one year post detonation NRDL reports: “. . In muscle and viscera samples of the red =r NRDL veys,? and Tables 26 and 27 for the July 1956 survey.’ In two pools of 15 and 19 fish muscle samples collected in late July 1956 and analyzed * No detectable activity. HA8SL Tables 24 and 25 show the radiochemical analyses made by AFL for the 1954-55 sur- Sr contributes approximately 0.5 percent of the total beta activity. Sr” is present in an approximately 1:1 ratio with Sr®. Since the Hunter and Ballou calculations indicate that Sr® and Sr” each contribute about 2 percent of the total beta activity at one year after fission, there does not appear to be any fractionation of radiostrontium into the soft tissues. As expected, most of the internally deposited radioactivity was found in the skeleton. “Tissues of a few marine specimen were analyzed for Cs'** (37-year half-life)* since this nuclide was present in high concentrations in water and coconut milk from this area. The tissues of the rooster and of the coconut crab contein significant amounts of Cs’, A very high fraction of Cs"activity was noted in the "Nowest estimates indicate 27,7-year half-life, muscle of the rooster (40 percent of the total beta).* Further radioanalyses of marine specimens indicated that the rare earth group constituted 2 few percent of the total beta activity. Ru-Rh'and Zr®*-Nb"contributed the largest percentage of the total beta activity.” The AFL reports: “. . « The Sr values for food plants, except coconuts, collected in October 1955 approximate the theoretical proportion of mixed fission products activity? ot 1.7 years, 4 percent. Coconuts contained 0.1 percent Sr with appropriate correction for timeof collection. . . . “.. Ia contrast to the strictly marine forms, the coconut crab, which feeds principally on land plants, had Srlevels of 3 percent in the muscle and 12 percent in the hepatopancreas or liver, where calcium salts are stored. The radioisotopes in salts leached from the carapace were found to consist entirely of Sr “. . . Radionuclides of Sr, Os, Ce and their daughters did not account for the total activity in most (fish) samples analyzed. Complete fission product analyses of samples collected at Eniwetok and Bikini Atolls indicate that non-fission-product radionuclides may account for more than half of the total activity in some fish. Zn contributes one-fourth or more of the total activity in shark muscle as determined by radiochemical analysis and confirmed by following the decay.’ (Zn is not a fission product.) The two-year survey by NRDL continues to indicate the high percentage of Zn® in fish. *See Section IV. 23

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