is indicative of greater soil water content during the 1965 measurement period compared to that of 1962 and 1963. These areas experienced greatly increased rainfall during the previous year or so while the Northeast experienced drought conditions. During the 1962 and 1963 surveys extremely dry and dusty conditions were prevalent over much of this area. The Denver area, in particular, experienced widespread flooding during the spring of 1965. This increased moisture is reflected in the Denver data (Table IV). The effect of moisture in the soil on dose rates and spectrometric dose rate measurements is being studied in some detail. (See Section IV.) While the major fallout contributors to the gamma dose rate in 1962 and 1963 were 9°9zr -— 95Nb and 106pn, the major contributors during 1965 were 137cs, 196Rh and 54mn with traces of 125sb and 144ce - 144pr detectable at almost all soil locations. Studies of Cosmic Ray Ionization In order to study cosmic ray ionization as a function of altitude spectra were obtained over a number of large lakes at various altitudes up to 10,000 feet. These results are given in Table V. The measurements at Red Mountain and at an open pit asbestos mine near Copperopolis, California shown in Table V are considered as cosmic ray measurements and treated with the lake measurements since the serpentine rock at both these locations exhibited very little gamma activit The 4" x 4" detector was placed in its stand as used in the field facing downward® at one end of a small aluminum or fiberglass boat. In all cases measurements were made more than 1/2 mile from shore to minimize interference from gamma emitters in the soil. All of the spectra indicated the presence of some gamma activity. Two representative cosmic ray ionization spectra are shown in Figure 2. The only significant gamma contributors were radon daughters in the air. As shown in Table V our estimates of the gamma dose rate from the spectra range between 0.1 ur/hr and 0.5 ur/fhr. Using these gamma dose rates we have estimated for each lake spectrum the total "energy" in the band 0.15 MeV to 3.4 MeV due to cosmic ray secondaries. The cosmic ray response for each of the three - 10 -

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