760 MARTIN Herbivorous mammals may be externally contaminated by direct exposure to fallout or by contact with contaminated plants or soils. Radionuclides may accumulate in animal tissues via inhalation, which, in many cases, is relatively unimportant or via ingestion of contaminated materials. Although inhalation, ingestion of contaminated soil or water, and ingestion of fallout particles while the animal is preening cannot be dismissed entirely, it is probably reasonable to assume that externally contaminated plants are the major sources of radionuclides for assimilation by herbivorous mammals (e.g., jackrabbits or dairy cattle) feeding in a fallout-contaminated environment during the first 30 to 90 days after close-in fallout. The summer of 1962 provided an excellent opportunity to study the food-chain kinetics of Sr and ‘I in relation to desert shrubs and rabbits in the Sedan fallout field. These studies included the formulation and testing of mathematical models that can be shown to provide at least a partial explanation of the kinetic relations between initial concentrations of Sr and '!I on fallout-contaminated plants and sub- sequent concentrations of ®Sr in the bone ash or of '*I in the thyroids of rabbits collected in the Sedan fallout field. Although the results of these studies!!~!’ are not conclusive, partly because the causes of vari- ation are imperfectly understood, they do provide evidence that math- ematical models similar to those used by radiochemists to explain decay-chain kinetics,'® by physiologists to explain tracer kinetics,'® and by the International Commission on Radiological Protection (ICRP) to establish maximum permissible concentrations’’ can also be used to study food-chain kinetics under field conditions. The objectives of this paper are (1) to summarize someof the data related to ™Sr and "I on desert shrubs and in rabbit tissues following fallout from Project Sedan, (2) to present the deterministic models that provide a partial explanation of these results, and (3) to illustrate the potential value of similar models in studying the food-chain kinetics of radionuclides on pasture plants, in cow milk, and in human tissues following a single fallout event. METHODS Project Sedan, a peaceful nuclear-explosives test, involved the detonation of a 100 + 15 kt thermonuclear device at a depth of 635 ft in alluvium and tuff at the north end of the Nevada Test Site on July 6, 1962. As predicted, the early fallout was relatively light and occurred primarily within a 150-mile sector, N60°W to N60°E, from ground zero in Yucca Flat. Before and at various times after the detonation, plant samples and rabbits were collected from representative locations in the Sedan fallout field (see Fig. 2). Each sampling station was marked by a metal

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