PREDICTION OF RADIONUCLIDE DEPOSITION ‘10° Se = _N Y .a er Sie = E & 4 °° SE? -F O ; a be a ee TTI TUTTO a be ©4 731 TY 7 ) 7 8 4 a = 5 CB 3 eo o a o 4 pede te te tia ft pal cual ply 1424 3/21 5/16 7/11 9/5 10/3112/26 2/20 4/16 6/11 + 1963 ma 1964 —o 4 9° Fig. 3—Comparison between the predicted (C) and the measured (A) depositions of gross beta radioactivity for four-week sampling periods at Tecumseh, Mich. DISCUSSION Admittedly, the model was used in an arbitrary fashion to predict the deposition on the Tecumseh farm. Itcertaiply ie unuesirable to have to keep the model current with an extensive program of measurements just to be able to predict the deposition at one location. In the following discussion an attempt is made to show that the model in its general form may be widely applicable. On the other hand, it will be shown that its applicability to specific situations is limited because at the present time the behavior of certain terms in the model cannot be predicted. Applicability First of all, with the model selected it was assumed that radioac- tivity is washed from the atmosphere exponentially with rainfall. Since the rainfall collected during a four-week period isthe sum of individual rainfalls, one might expect to find an exponential relation between the deposition and the amount of rainfall on, say, a daily basis. In the literature on this subject, the relation that is repeated again and again is the apparently logarithmic one between the radioactivity concentration in rain and the amount of daily rainfall. This relation has been reported in Norway® from 1956 to 1959, in Great Britain’ in 1956 and 1957, and in Russia.’ The period during which the relation was found in Russia was not reported, but it probably was in 1960 and/or 1961. Figure 4 shows the relation plotted logarithmically. The points in Fig. 4 were determined by dividing the daily rain concentrations by their respective monthly concentration, averaging the data over several months Td of

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