668 THATCHER, PAYNE, AND CAMERON The North American continent provides the opportunity to study a meridional traverse over an essentially continental environment, just as the Pacific provided the same traverse for an oceanic environment. Data for Fort Smith (CR), Edmonton (CR), Chicago (IA), and Flagstaff (IA) are averaged for the full year of 1963. Station Fort Smith Edmonton Chicago Flagstaff Location Mean T.U. 60°01’N, 111°58’W 3836 35°12/N, 111°40’W 1471 53°34’N, 113°31'W 41°47/N, 87°44°W 4193 2333 The tritium concentrations increase toward the north. However, it is not certain that this is solely a latitude effect. The difference between the Canadian and U. S. sites must be attributed in part, at least, to the effect of oceanic air from the Gulf of Mexico; therefore it is not entirely a latitude effect. In other parts of the world, sites south of Chicago have shown higher tritium averages. Teheran (35°41'N) averaged 3150 T.U. for the first half of 1963, com- pared to 2333 T.U. for Chicago. Presumably, Teheran is less affected by oceanic air masses than is Chicago and is therefore more truly representative of a continental site at this latitude. Data for eastern North America (IA, GS) are given in Fig. 9, showing an increasing oceanic component from Hatteras, N. C., to Ocala, Fla. Data from South America are incomplete, partly because of the poor cooperation of national authorities. Large parts of Brazil remain unsampled. Data from Buenos Aires indicate that higher tritium concentrations may be developing in South America, possibly because of high-altitude interception by the Andes. The March 1964 measurement of Buenos Aires rain (IA) was 110 T.U., and the April measurement was 86 T.U. In the Falkland Islands relatively high concentra- tions were measured in 1964 as follows (IA): January, 42 T.U.; February, 29 T.U.; March, 43 T.U.; and April, 18 T.U. RATIO OF TRITIUM TO 9°Sr IN PRECIPITATION The fractionation of tritium from particulate fallout in the course of global circulation may be observed by comparing tritium and "Sr deposition at selected sites. As a gaseous molecule, the transport phenomena for tritium are not identical with the transport phenomena for Sr, and the investigation of these differences should lead toa better understanding of the transport mechanisms. The relation be- tween HTO and “Sr deposition may be observed in Figs. 11 and 12 for typical northern-hemisphere and southern-hemisphere sites, respectively.

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