40 FREILING, CROCKER, AND ADAMS ACKNOWLEDGMENTS We are most grateful to Col. Irving J. Russell of the Air Force Weapons Laboratories and Dr. John Norman of General Atomic DiviSion, General Dynamics Corporation, for permission to present their data prior to publication. APPENDIX TERMS AND DEFINITIONS RADIONUCLIDE FRACTIONATION Any alteration of radionuclide composition occurring between the time of detonation and the time of radiochemical analysis which causes the debris sample to be nonrepresentative of the detonation products taken as a whole. FRACTIONATED Two substances, either radionuclides or inert ma- terial, are fractionated with respect to each other in a sample of debris if they are not present in their representative ratio. The term is meaningless when applied to a single substance. *POTENTIAL FRACTIONATION The existence of different composi- tions in various portions of a sample of debris when these portions are subject to separation by subsequent natural processes, é.g., the existence of particles of different size with different compositions in the same portion of a nuclear cloud or of a slurry in which different nuclides are distributed between liquid and solid phases in different proportions. *NATURAL FRACTIONATION Fractionation produced by the processes occurring subsequent to detonation. *PRIMARY FRACTIONATION IN AIR, TOWER, AND SURFACE BURSTS Actual fractionation produced by meteorological, gravitational, and centrifugal separation of potentially fractionated particles in a cloud. *SECONDARY FRACTIONATION IN AIR, TOWER, AND SURFACE BURSTS Fractionation produced by interaction of the debris with radioactively inert environment (e.g., leaching with water or pref- erential small particle adsorption on surfaces). *ARTIFACTITIOUS FRACTIONATION Fractionation resulting from human intervention (e.g., biased sampling, incomplete decontami- nation of collector surfaces, and faulty analytical techniques). FRACTION OF CONSITITUENT OR EXTENSIVE PROPERTY IN A SAMPLE The ratio of the quantity of said constituent or property to the total amount produced by the device and measured at the same time whennecessary (replaces the “bomb-fraction” concept). * Asterisks indicate convenient, but not essential, terms.

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