VARIATION OF RADIOACTIVITY IN SURFACE AIR 499 > 1peril 3 Ltatil "Cs ae < rm | TTT 107! hd a Cc ~ TTT JUNE APRIL 107 ta diitul TTT Wes, eh, AND Mn, PC/SCM 3 z= x 1 il IB EADODAROD ROORERORROED LRROROU ACRE RERORER ORD EARRRRRSREEERRORRDROED 2 ‘ J é = 4 ~ Trim 1073 4 ' U.S.S.R. TESTS 4 U.S. TESTS ‘ouees SERRUCEUBERREUUSECREGESEEREREER SHORE SREEREGHEGUROCRUGHUUNEHOGRUGEEEEEEE Jan.— Dec. 1959 Jan.— Dec. 1960 Jan.— Dec. 1961 Jan.— Dec. 1962 Jan.— Dec. 1963 Jan.— Dec. 1964 Fig. 1—1%"Cs, !"Rh, and 54Mn in surface air at Argonne, Ill. each year. In 1961 the maximum was observed during May and June, and in 1962 and 1963, during June and July. In 1964 the maximum occurred during late May and early June, as indicated in Fig. 1. Similar observations have been made at other locations within the northern hemisphere.>~> During 1961 through mid-1964, an appreciable portion of the total 137Cg present in surface air was of high-altitude origin as inferred from the measured concentrations of ‘"Rh and *Mn, which are also illustrated in Fig. 1. The !"*Rh was produced for the most part as a tracer in the Orange shot of the Operation Hardtack I test series on Aug. 11, 1958, which had a burst height of about 43 km over Johnston Island.® The concentrations of '*Rh have been corrected for radioactive decay to that date. Manganese-54 was produced inhigh-yield shots dur- ing the Soviet 1961 test series, and there are indications from the Ash Can balloon flights made at San Angelo, Tex.,’:® that “Mn was also pro- duced during high-yield and/or high-altitude shots during 1962. The *4Min values shown in Fig. 1 have been corrected for radioactive decay to mid-October 1961. Thus both !°*Rh and *4Mn may be reasonably used as tracers for high-altitude debris. As seen in Fig. 1, '*Rh reached a

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