242 LOWDER, BECK, AND CONDON close. The decline in late 1963 is quite striking. It should be noted that the differences in the various natural-gamma readings are at least partly real. For example, the low reading in April 1964 was obtained when the ground was quite wet. This would tend to reduce all components to some extent. Rainfall can have a significant effect on both the total observed fallout dose rates and on how well they can be determined. This is exemplified by our October 1962 measurements on the Olympic Peninsula in the state of Washington, given in Table 4. Over a distance of 50 Table 4 MEASUREMENTS ON THE OLYMPIC PENINSULA, WASHINGTON, OCTOBER 1 AND 2, 1962 Mean annual rainfall, in.* Town Sequim Sequim Port Angeles Port Angeles Joyce 14 14 24 24 54 Clailam Bay 81 Forks 118 Forks Forks 118 118 - Gamma dose rates, ur/hr Sr, me/sq milet 42.0 65.3 84.1 133 153 %57r—®5Nb Natural Total Fallout 1t Fallout 2§ 1.2 1.4 1.0 0.9 0.8 0.6 0.8 1.1 1,0 1.8 3,3 3.8 3.5 3.2 3.7 0.8 1.1 1.4 1.3 2.4 0.7 14 1.7 1.5 1.3 “K "87 282yh 1.2 1.5 1.6 1.2 1.7 0.9 0,9 0.9 1.1 1.2 1.9 17 2.2 1.3 0.4 2.2 2.7 5.2 3.4 2.8 2.6 1.5 1.1 1,7 1.1 1.2 0.9 2.5 2.3 4.4 3.1 3,7 3.4 2.8 2.8 1.3 2.6 2.7 *1960—1962 value. +Oct. 1-2, 1962, soil determinations (L. T. Alexander). tFrom photopeak calibrations. , § From total terrestrial] dose-rate measurements with natural component subtracted. miles from east (Sequim) to west (Forks), the mean annual rainfall increases by a factor of nearly 10. This was strikingly illustrated for us at Forks by the soggy condition of the ground, the mist in which we made our measurements, and the two sudden downpours that nearly put a permanent end to our survey. The strong increase in the falloutgamma levels with mean annual rainfall is clear from the table, as is the poorer agreement between our two methods for estimating these levels at Forks than at the other locations. The latter phenomenon can be explained as the effect of recent deposition of significant quantities of fission products, particularly *Zr—*Nb, forming a more nearly plane source than our theory assumes and thus resulting in an overestimate of the dose rate from the peak method. The presence of the . short-lived °Ba—'°La peaks in our Forks spectra provides further evidence of recent deposition. Our survey results taken as a whole indicate that, until late in 1963, *Zr—*Nb contributed 60 to 80% of the observed fallout-gamma dose rate in the environment and that these dose rates were of the order of 50% of the natural levels at typicallocations over open ground. By one year after the last nuclear weapons tests in December 1962, these levels had fallen to 10 to 20% of the average natural-gamma dose

Select target paragraph3